化工进展 ›› 2024, Vol. 43 ›› Issue (5): 2786-2802.DOI: 10.16085/j.issn.1000-6613.2023-1584
• 二氧化碳捕集与资源化利用 • 上一篇
收稿日期:
2023-09-07
修回日期:
2023-12-22
出版日期:
2024-05-15
发布日期:
2024-06-15
通讯作者:
詹国武
作者简介:
卢欣欣(1998—),女,硕士研究生,研究方向为集成催化剂。E-mail:lxx_18960186016@163.com。
基金资助:
LU Xinxin(), CAI Dongren, ZHAN Guowu(
)
Received:
2023-09-07
Revised:
2023-12-22
Online:
2024-05-15
Published:
2024-06-15
Contact:
ZHAN Guowu
摘要:
针对催化剂活性位点和微观结构不可控的问题,采用固体前体作为缓释的金属离子源制备微观结构可控、活性位点空间位置明确的金属基集成催化剂有望解决该问题,并实现催化剂的定制化设计。本文介绍了4类固体前体材料用于制备CO2热催化加氢反应的催化剂,包括过渡金属层状硅酸盐、层状双金属氢氧化物、金属有机骨架材料以及钒酸铋材料。总结了这4类集成催化材料的制备过程机制及其在CO2热催化加氢中的应用实例,并对固体前体制备多组分集成催化剂的研究前景进行了展望。
中图分类号:
卢欣欣, 蔡东仁, 詹国武. 基于固体前体构建集成催化剂及CO2加氢研究进展[J]. 化工进展, 2024, 43(5): 2786-2802.
LU Xinxin, CAI Dongren, ZHAN Guowu. Research progress in the construction of integrated catalysts based on solid precursors and their application in CO2 hydrogenation[J]. Chemical Industry and Engineering Progress, 2024, 43(5): 2786-2802.
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