CO2应用于油砂处理的工艺进展

doi:10.16085/j.issn.1000-6613.2023-1629

化工进展 ›› 2024, Vol. 43 ›› Issue (10): 5569-5580.DOI: 10.16085/j.issn.1000-6613.2023-1629

• 材料科学与技术 • 上一篇

CO₂应用于油砂处理的工艺进展

徐壮壮¹(), 季程程²(), 于斌¹, 程思远³, 艾小茜⁴, 杨双春¹

^1.辽宁石油化工大学石油天然气工程学院，辽宁抚顺 113001
^2.辽宁石油化工大学实训中心，辽宁抚顺 113001
^3.辽宁石油化工大学国际教育学院，辽宁抚顺 113001
^4.辽宁石油化工大学石油化工学院，辽宁抚顺 113001

收稿日期:2023-09-14 修回日期:2023-12-05 出版日期:2024-10-15 发布日期:2024-10-29
通讯作者: 季程程
作者简介:徐壮壮（1998—），男，硕士研究生，研究方向为油气井工程。E-mail：15668554951@163.com。
基金资助:
辽宁省教育厅应用研究一般项目(LJKZ0393);辽宁省科技厅应用基础研究一般项目(2023JH2)

Research progress of CO₂ application on oil sands treatment

XU Zhuangzhuang¹(), JI Chengcheng²(), YU Bin¹, CHENG Siyuan³, AI Xiaoxi⁴, YANG Shuangchun¹

^1.College of Petroleum and Natural Gas Engineering, Liaoning Petrochemical University, Fushun 113001, Liaoning, China
^2.Engineering Training Centre, Liaoning Petrochemical University, Fushun 113001, Liaoning, China
^3.College of International Education, Liaoning Petrochemical University, Fushun 113001, Liaoning, China
^4.College of Petrochemical Technology, Liaoning Petrochemical University, Fushun 113001, Liaoning, China

Received:2023-09-14 Revised:2023-12-05 Online:2024-10-15 Published:2024-10-29
Contact: JI Chengcheng

摘要/Abstract

摘要：

油砂作为一种储量丰富的非常规石油资源，越来越受到世界各国的广泛关注，油砂处理行业和生态环境的协调可持续发展也已成为亟需解决的热点问题。因此，为了建构清洁低碳、节能高效的工艺流程体系，促进油砂处理行业的高质量发展，对CO₂在油砂处理中的工艺发展形成全局性的认识，本文重点总结了国内外研究CO₂在油砂处理中的应用现状以及对CO₂在油砂处理上的数值模拟和动力学模拟概况进行了综述。其中，重点论述了CO₂响应作用下分离油砂、超临界CO₂萃取油砂以及CO₂在其他工艺中的应用现状。但是，目前的研究仅限于室内，而且工业化试验的数据相对较少，这限制了我国油砂处理行业的工业化应用。因此还需要对CO₂在油砂处理中的工艺进行更加深入的研究，以满足工业化应用的要求。最后，对CO₂在油砂处理的应用进行了总结与展望。

关键词: 二氧化碳, 萃取, 油砂处理, 尾矿处理, 动力学模拟, 数值模拟

Abstract:

As a kind of unconventional oil resource with abundant reserves, oil sands have attracted more and more attention from all over the world. The coordinated and sustainable development of oil sands treatment industry and ecological environment has become a hot issue that needs to be solved urgently. Therefore, in order to construct a clean, low-carbon, energy-saving and efficient process system and promote the high-quality development of the oil sand treatment industry, the process development of CO₂ in oil sand treatment has formed a global understanding. The application status of CO₂ in oil sand treatment at home and abroad, as well as the numerical simulation and kinetic simulation of CO₂ in oil sand treatment were summarized. Among them, the separation of oil sands under the action of CO₂ response, supercritical CO₂ extraction of oil sands and the application of CO₂ in other processes were mainly discussed. However, the current research is limited to indoors, and the data of industrial test was relatively small, which inevitably limited the industrial application of China's oil sand treatment industry. Therefore, more in-depth research on the process of CO₂ in oil sand treatment was needed to meet the requirements of industrial application. Finally, the application of CO₂ in oil sand treatment was summarized and prospected.

Key words: carbon dioxide, extraction, oil sands treatment, tailings treatment, kinetic simulation, numerical simulation

中图分类号:

TQ028.8

徐壮壮, 季程程, 于斌, 程思远, 艾小茜, 杨双春. CO₂应用于油砂处理的工艺进展[J]. 化工进展, 2024, 43(10): 5569-5580.

XU Zhuangzhuang, JI Chengcheng, YU Bin, CHENG Siyuan, AI Xiaoxi, YANG Shuangchun. Research progress of CO₂ application on oil sands treatment[J]. Chemical Industry and Engineering Progress, 2024, 43(10): 5569-5580.

图/表 13

图1 复合可切换水水洗油砂工艺流程[16]

图2 CO2作用下不同类型的SFME微乳液pH变化图

图3 CO2作用下不同类型的SFME微乳液电导率变化图

图4 微乳液洗过模拟油砂废液在通入CO2前后的外观变化照片[23]

图5 微乳液洗过工业油砂废液在通入CO2前后的外观变化照片[23]

图6 鼓泡分离法去除萃余砂中残留溶剂的分离机理示意图[28]

图7 CyNMe2萃取油砂沥青工艺流程[29]

图8 新型重质油矿溶剂萃取分离工艺流程示意图[30]

图9 超临界CO2萃取含油泥砂工艺流程图[33]

图 10 实验设备流程图[46]（测试流体由两台Q5000排量泵加压）

图11 在MFT中引入CO2的各种方法[57]

图12 三维分子结构模型[61]

图13 甲苯-水-CO2体系结构示意图[63]

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CO₂应用于油砂处理的工艺进展

Research progress of CO₂ application on oil sands treatment

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