化工进展 ›› 2022, Vol. 41 ›› Issue (5): 2441-2450.doi: 10.16085/j.issn.1000-6613.2021-1256
薛李静(), 费星, 刘江淋, 吴林军, 仇中杰, 许权洲, 钟晓文, 林绪亮(
), 秦延林(
)
收稿日期:
2020-06-16
修回日期:
2021-08-25
出版日期:
2022-05-05
发布日期:
2022-05-24
通讯作者:
林绪亮,秦延林
E-mail:2112006138@mail2.gdut;xllin@gdut.edu.cn;ylqin@gdut.edu.cn
作者简介:
薛李静(1997—),女,硕士研究生,研究方向为木质素基碳材料的制备及应用。E-mail: 基金资助:
XUE Lijing(), FEI Xing, LIU Jianglin, WU Linjun, QIU Zhongjie, XU Quanzhou, ZHONG Xiaowen, LIN Xuliang(
), QIN Yanlin(
)
Received:
2020-06-16
Revised:
2021-08-25
Online:
2022-05-05
Published:
2022-05-24
Contact:
LIN Xuliang,QIN Yanlin
E-mail:2112006138@mail2.gdut;xllin@gdut.edu.cn;ylqin@gdut.edu.cn
摘要:
木质素具有三维网状苯环结构、来源丰富、含碳量高、官能团丰富可控等特点,是一种理想的碳材料前体。通过化学改性和微结构调控制备具有特殊功能的木质素基碳材料,其在能源催化转化、电化学储能和环境修复等领域应用广泛。本文介绍了木质素基碳材料催化剂的国内外最新研究进展,总结了木质素基碳材料催化剂的制备方法,重点综述了木质素基碳材料催化剂在氧化反应、氢解反应、酯化反应、水解反应、脱水反应、费托合成等热催化反应、电解水析氢和锌空气电池氧还原等电催化反应、有机污染物降解等光催化反应的研究进展,但如何构筑高效、稳定、廉价、可规模生产的木质素基碳材料催化剂仍然是一个具有挑战性的课题。文章总结:今后研究中应加强对木质素的基础化学结构和微结构调控、活性组分与木质素碳材料载体间的相互作用、木质素基碳材料催化剂在催化反应中的作用机理等的研究,更好地发挥其低成本、三维结构易成型和微结构可调控等优势,拓展木质素生物质资源的高值化利用领域。
中图分类号:
薛李静, 费星, 刘江淋, 吴林军, 仇中杰, 许权洲, 钟晓文, 林绪亮, 秦延林. 木质素基碳材料催化剂的制备及应用研究进展[J]. 化工进展, 2022, 41(5): 2441-2450.
XUE Lijing, FEI Xing, LIU Jianglin, WU Linjun, QIU Zhongjie, XU Quanzhou, ZHONG Xiaowen, LIN Xuliang, QIN Yanlin. Research progress on the preparation and application of lignin-based carbon catalysts[J]. Chemical Industry and Engineering Progress, 2022, 41(5): 2441-2450.
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