化工进展 ›› 2023, Vol. 42 ›› Issue (5): 2691-2701.DOI: 10.16085/j.issn.1000-6613.2023-0055

• 资源与环境化工 • 上一篇    下一篇

木质纤维类废弃物定向生物转化乳酸、乙酸研究进展

黄越1,2(), 赵立欣2, 姚宗路2, 于佳动2(), 李再兴3, 申瑞霞2, 安柯萌1,2, 黄亚丽1   

  1. 1.河北科技大学环境科学与工程学院,河北 石家庄 050018
    2.中国农业科学院农业环境与可持续发展研究所,农业农村部华北平原农业绿色低碳重点实验室,北京 100081
    3.北京石油化工学院环境工程系,北京 102617
  • 收稿日期:2023-01-12 修回日期:2023-02-07 出版日期:2023-05-10 发布日期:2023-06-02
  • 通讯作者: 于佳动
  • 作者简介:黄越(2000—),女,硕士研究生,研究方向为农业废弃物厌氧发酵工艺。E-mail:haungyue20000504@163.com
  • 基金资助:
    国家重点研发计划(2022YFD2002102);中国农业科学院科技创新工程项目;中央级公益性科研院所基本科研业务费专项(BSRF202204)

Research progress in directed bioconversion of lactic acid and acetic acid from wood lignocellulosic wastes

HUANG Yue1,2(), ZHAO Lixin2, YAO Zonglu2, YU Jiadong2(), LI Zaixing3, SHEN Ruixia2, AN Kemeng1,2, HUANG Yali1   

  1. 1.School of Environmental Science and Engineering, Hebei University of Science and Technology, Shijiazhuang 050018, Hebei, China
    2.Institute of Environment and Sustainable Development in Agriculture, Chinese Academy of Agricultural Sciences, Key Laboratory of Low-carbon Green Agriculture in North China, Ministry of Agriculture and Rural Affairs, PRC,Beijing 100081, China
    3.Department of Environmental Engineering, Beijing Institute of Petrochemical Technology, Beijing 102617, China
  • Received:2023-01-12 Revised:2023-02-07 Online:2023-05-10 Published:2023-06-02
  • Contact: YU Jiadong

摘要:

依托厌氧发酵技术处理秸秆和牛粪等木质纤维类废弃物,是资源循环利用的重要方式之一。乳酸和乙酸是厌氧发酵的重要中间产物,是生产沼气、中链脂肪酸等能源化工产品的重要前体物质,但定向生物转化协同生产效率不高、对木质纤维类废弃物协同产乳酸、乙酸机制等问题有待深入探索。本文基于对产酸代谢途径机理的分析,梳理了同步发酵和分步发酵协同产乳酸、乙酸特性,归纳了影响生物转化产酸效率的关键因素,发现在较高含固率15%~20%、接种20%~40%的活性物质和适宜的过程参数[pH为5.0左右、中温和有机负荷5~10kgVS/(m3·d)]下,木质纤维类废弃物具有良好的协同产酸效果。进一步探明物化和生物强化耦合手段对木质纤维素降解和目标产物的促进效应,为开发生物转化乳酸、乙酸协同生产关键技术以及促进秸秆等木质纤维类废弃物高值转化利用提供理论依据。

关键词: 乳酸, 乙酸, 厌氧发酵, 协同产酸, 中链脂肪酸, 木质纤维类废弃物

Abstract:

Anaerobic fermentation technology is one of the critical ways of resource recycling to treat wood lignocellulosic wastes such as straw and cow manure. Lactic acid and acetic acid are essential intermediate products of anaerobic fermentation, and significant precursor substances for the production of biogas, medium chain fatty acids and additional energy chemical products. However, the collaborative production efficiency of directed biotransformation is not elevated, and the mechanism of collaborative production of lactic acid and acetic acid from wood lignocellulosic waste still needs to be further explored. Based on the analysis of the metabolic pathway mechanism of acid production, this paper sorted out the characteristics of simultaneous fermentation and stepwise fermentation in collaborative production of lactic acid and acetic acid and summarized the key factors affecting the efficiency of biological transformation in acid production. It was found that the wood lignocellulosic waste had a favorable synergic acid production effect under high solid content of 15%—20%, inoculation of 20%—40% active substances and appropriate process parameters [pH=5.0, moderate temperature and moderate organic load 5—10kgVS/(m3·d)]. In addition,we explored the promoting effect of physicochemical and bio strengthening coupling means on lignocellulosic degradation and target products, which provided a theoretical basis for the development of key technologies for the collaborative production of lactic acid and acetic acid by bioconversion, and the promotion of high-value conversion and utilization of wood lignocellulosic waste such as straw.

Key words: lactic acid, acetic acid, anaerobic fermentation, co-production of acid, medium chain fatty acid, wood lignocellulosic waste

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