二维材料纳米油墨的制备及喷墨打印研究进展

doi:10.16085/j.issn.1000-6613.2023-0833

摘要/Abstract

摘要：

以石墨烯为代表的二维材料具有出色的综合性能，可用其制作功能纳米油墨，通过喷墨打印可加工得到光电功能器件，其在能源、环境、生命健康等领域具有广阔的应用前景。本文总结了几种典型二维材料的性能、其纳米油墨的制备及喷墨打印应用等，重点介绍了液相剥离和喷墨打印过程的调控。对比不同剥离方法及原理，并对喷墨打印相关理论如咖啡环效应、马兰戈尼效应等进行综述。指出可通过对二维材料剥离过程及其纳米油墨打印过程的精准调控，形成基于喷墨打印的先进微纳制造技术，实现不同功能微纳电子元件和器件的低成本加工，推动生物传感、柔性电子等领域的发展。

关键词: 二维材料, 液相剥离, 纳米油墨, 喷墨打印, 电子器件

Abstract:

Two-dimensional materials represented by graphene possess excellent comprehensive performance, which can be used to manufacture functional nano-inks and obtain optoelectronic functional devices by ink-jet printing. There are broad application prospects in the fields of energy, environment, life and health. This paper systematically summarized the properties of several typical two-dimensional materials, the preparation of nano-inks and the application of ink-jet printing, focusing on the regulation of liquid phase exfoliation and ink-jet printing processes. Different exfoliation methods and principles were summarized and compared, as well as the related theories of ink-jet printing, such as the coffee ring effect and Marangoni effect, were reviewed. Through the precise regulation of the two-dimensional material exfoliation process and its nano-inks printing process, it was expected to form an advanced micro-nano manufacturing technology based on ink-jet printing, realize the low-cost processing of different functional micro-nano electronic components and devices, and promote the development of biosensing, flexible electronics and other fields.

Key words: two-dimensional material, liquid-phase exfoliation, nano-inks, ink-jet printing, electronic device

中图分类号:

TQ11

张妤欣, 黄孝东, 陈迪, 邓杭军, 王文俊, 刘平伟. 二维材料纳米油墨的制备及喷墨打印研究进展[J]. 化工进展, 2024, 43(6): 3145-3158.

ZHANG Yuxin, HUANG Xiaodong, CHEN Di, DENG Hangjun, WANG Wenjun, LIU Pingwei. Progress in the preparation and ink-jet printing of 2D material-based nano-inks[J]. Chemical Industry and Engineering Progress, 2024, 43(6): 3145-3158.

图/表 4

图1 广义液相剥落机理示意图[47]

图2 喷墨打印设备工作原理示意图[78]

图3 环状染色和产生这种染色的物理过程演示[83]

图4 辛烷液滴烘干过程的液体流场[88]（Ma=48000，明显的马兰戈尼旋涡）

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