化工进展 ›› 2023, Vol. 42 ›› Issue (2): 624-630.DOI: 10.16085/j.issn.1000-6613.2022-1704

• 专栏:工业污泥/精馏釜残的热化学转化利用 • 上一篇    下一篇

改性Au-TiO2光降解废水中诺氟沙星的影响

多佳1(), 姚国栋2, 王英霁3, 曾旭2, 金滨滨4()   

  1. 1.中国科学院新疆生态与地理研究所,新疆维吾尔自治区环境污染与生态修复重点实验室,新疆 乌鲁木齐 830011
    2.同济大学环境科学与工程学院,污染控制与资源化研究国家重点实验室,上海 200092
    3.中国科学院新疆理化技术研究所,新疆 乌鲁木齐 830011
    4.上海交通大学环境科学与工程学院,上海 200240
  • 收稿日期:2022-09-13 修回日期:2022-11-23 出版日期:2023-02-25 发布日期:2023-03-13
  • 通讯作者: 金滨滨
  • 作者简介:多佳(1980—),女,博士,助理研究员,研究方向为干旱区有机污染防治技术、生态修复。E-mail:duojia2017@ms.xjb.ac.cn
  • 基金资助:
    国家重点研发计划(2018YFC1902103);2017年自治区高层次人才引进项目(Y846011)

Effects on the photo-degradation of norfloxacin using modified Au-TiO2

DUO Jia1(), YAO Guodong2, WANG Yingji3, ZENG Xu2, JIN Binbin4()   

  1. 1.Xinjiang Key Laboratory of Environmental Pollution and Bioremediation, Xinjiang Institute of Ecology and Geography, Chinese Academy of Sciences, Urumqi 830011, Xinjiang, China
    2.State Key Laboratory of Pollution Control and Resources Reuse, College of Environmental Science and Engineering, Tongji University, Shanghai 200092, China
    3.Xinjiang Technical Institute Physics and Chemistry, Chinese Academy of Sciences, Urumqi 830011, Xinjiang, China
    4.School of Environmental Science and Engineering, Shanghai Jiao Tong University, Shanghai 200240, China
  • Received:2022-09-13 Revised:2022-11-23 Online:2023-02-25 Published:2023-03-13
  • Contact: JIN Binbin

摘要:

诺氟沙星作为喹诺酮类抗生素的一种,被广泛用于医疗、畜牧业、农业和水产养殖等行业,大量抗生素的生产、使用和非法排放造成水环境中抗生素污染问题日益突出,对生态系统和人类健康构成潜在的危害。而目前现有的抗生素的去除方法效率有限,本文制备了Au-TiO2光催化剂,重点研究了水中酸碱度、氯离子浓度及Au-TiO2催化剂量对Au-TiO2光催化剂可见光降解诺氟沙星的影响,获得最高80.7%的诺氟沙星的降解率。本研究不仅证明了Au-TiO2可见光高效降解诺氟沙星是可行的,也进一步表明了可见光催化技术处理抗生素废水是一种有应用潜力的方法。

关键词: Au-TiO2, 可见光催化, 降解, 诺氟沙星

Abstract:

Norfloxacin as one of quinolone antibiotics is widely used in medical treatment, animal husbandry, agriculture, aquaculture and other industries. In recent years, the accumulation of quinolones in the environment poses a direct or potential threat to ecosystem stability, diversity and human health. Therefore, how to rapidly degrade quinolones has become an urgent problem. However, the removal efficiency of the antibiotics is limited. Therefore, in this paper, the Au-TiO2 photocatalyst was prepared, and the effects on the visible light degradation of norfloxacin were mainly studied by changing the reaction conditions such as pH, chloride concentration and Au-TiO2 amount, and the highest norfloxacin degradation rate of 80% of was obtained. This study not only proved that the visible light degradation of norfloxacin by Au-TiO2 was feasible, but also further indicated that the visible light catalytic technology was a potential method for the treatment of antibiotic wastewater.

Key words: Au-TiO2, visible-light photocatalysis, degradation, norfloxacin

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