Chemical Industry and Engineering Progress ›› 2019, Vol. 38 ›› Issue (12): 5578-5586.DOI: 10.16085/j.issn.1000-6613.2019-0450
• Resources and environmental engineering • Previous Articles Next Articles
Deqian LIU1(),Qiang XIE1(),Chaoran WAN1,Feng DENG1,2,Xiaoqing HUANG1,ZHAI Xiaodi1
Received:
2019-03-26
Online:
2019-12-05
Published:
2019-12-05
Contact:
Qiang XIE
刘德钱1(),解强1(),万超然1,邓锋1,2,黄小晴1,翟笑迪1
通讯作者:
解强
作者简介:
刘德钱(1991—),男,博士研究生,研究方向为活性炭制备及应用。E-mail:基金资助:
CLC Number:
Deqian LIU,Qiang XIE,Chaoran WAN,Feng DENG,Xiaoqing HUANG,ZHAI Xiaodi. Adsorption properties of blending activated carbons and their relationship with pore structure[J]. Chemical Industry and Engineering Progress, 2019, 38(12): 5578-5586.
刘德钱,解强,万超然,邓锋,黄小晴,翟笑迪. 活性炭配炭的吸附性能及其与孔结构的关系[J]. 化工进展, 2019, 38(12): 5578-5586.
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编号 | M ad/% | A d/% | V daf/% | FCdaf/% |
---|---|---|---|---|
DT-830-BCT | 1.15 | 10.16 | 2.42 | 97.58 |
DT-830-DCT-1 | 0.53 | 13.40 | 1.48 | 98.52 |
DT-830-DCT-2 | 0.61 | 20.85 | 1.93 | 98.07 |
TX-830-ECT | 6.86 | 10.82 | 3.39 | 96.61 |
XJ-830-BCT | 1.29 | 7.29 | 2.00 | 98.00 |
XJ-830-DCT | 1.71 | 8.14 | 2.58 | 97.42 |
DT-830-DCT-3 | 0.75 | 18.53 | 1.93 | 98.07 |
DT-1240-BCT-1 | 2.81 | 8.84 | 2.64 | 97.36 |
DT-1240-DCT-1 | 3.49 | 14.02 | 2.58 | 97.42 |
DT-1240-DCT-2 | 0.95 | 20.17 | 2.28 | 97.72 |
DT-1240-BCT-2 | 4.09 | 13.70 | 2.96 | 97.04 |
编号 | M ad/% | A d/% | V daf/% | FCdaf/% |
---|---|---|---|---|
DT-830-BCT | 1.15 | 10.16 | 2.42 | 97.58 |
DT-830-DCT-1 | 0.53 | 13.40 | 1.48 | 98.52 |
DT-830-DCT-2 | 0.61 | 20.85 | 1.93 | 98.07 |
TX-830-ECT | 6.86 | 10.82 | 3.39 | 96.61 |
XJ-830-BCT | 1.29 | 7.29 | 2.00 | 98.00 |
XJ-830-DCT | 1.71 | 8.14 | 2.58 | 97.42 |
DT-830-DCT-3 | 0.75 | 18.53 | 1.93 | 98.07 |
DT-1240-BCT-1 | 2.81 | 8.84 | 2.64 | 97.36 |
DT-1240-DCT-1 | 3.49 | 14.02 | 2.58 | 97.42 |
DT-1240-DCT-2 | 0.95 | 20.17 | 2.28 | 97.72 |
DT-1240-BCT-2 | 4.09 | 13.70 | 2.96 | 97.04 |
编号 | 活性炭组成 | 质量比 | |
---|---|---|---|
AS-1 | DT-830-BCT | XJ-830-BCT | 7∶3 |
AS-2 | DT-830-BCT | XJ-830-BQ | 5∶5 |
AS-3 | DT-830-BCT | XJ-830-BCT | 3∶7 |
AS-4 | DT-830-BCT | DT-830-DCT-1 | 3∶7 |
AS-5 | DT-830-DCT-1 | DT-830-DCT-3 | 7∶3 |
AS-6 | DT-830-DCT-2 | XJ-830-DCT | 5∶5 |
AS-7 | DT-1240-BCT-1 | DT-1240-DCT-1 | 3∶7 |
AS-8 | DT-1240-BCT-1 | DT-1240-BCT-2 | 5∶5 |
编号 | 活性炭组成 | 质量比 | |
---|---|---|---|
AS-1 | DT-830-BCT | XJ-830-BCT | 7∶3 |
AS-2 | DT-830-BCT | XJ-830-BQ | 5∶5 |
AS-3 | DT-830-BCT | XJ-830-BCT | 3∶7 |
AS-4 | DT-830-BCT | DT-830-DCT-1 | 3∶7 |
AS-5 | DT-830-DCT-1 | DT-830-DCT-3 | 7∶3 |
AS-6 | DT-830-DCT-2 | XJ-830-DCT | 5∶5 |
AS-7 | DT-1240-BCT-1 | DT-1240-DCT-1 | 3∶7 |
AS-8 | DT-1240-BCT-1 | DT-1240-BCT-2 | 5∶5 |
吸附性能指标 | b 0 | b 1 | b 2 | R 2 |
---|---|---|---|---|
碘值 | 43.701 | 0.953 | 0.955 | 0.992 |
亚甲蓝值 | 0.0375 | 0.988 | 0.998 | 0.992 |
丹宁酸值 | -0.471 | 0.995 | 1.048 | 0.998 |
焦糖脱色率 | -0.0358 | 1.058 | 1.072 | 0.979 |
吸附性能指标 | b 0 | b 1 | b 2 | R 2 |
---|---|---|---|---|
碘值 | 43.701 | 0.953 | 0.955 | 0.992 |
亚甲蓝值 | 0.0375 | 0.988 | 0.998 | 0.992 |
丹宁酸值 | -0.471 | 0.995 | 1.048 | 0.998 |
焦糖脱色率 | -0.0358 | 1.058 | 1.072 | 0.979 |
吸附性能指标 | b 11 | b 22 | b 12 | b 10 | b 20 | b 00 | R 2 |
---|---|---|---|---|---|---|---|
碘值 | 3.287×10-5 | 2.639×10-5 | 5.590×10-5 | 0.895 | 0.903 | 70.001 | 0.992 |
亚甲蓝值 | -0.0011 | -0.0010 | -0.0023 | 1.407 | 1.395 | -37.326 | 0.992 |
丹宁酸值 | 0.0018 | -9.140×10-6 | 0.0015 | 0.932 | 1.038 | -0.138 | 0.997 |
焦糖脱色率 | -0.0109 | 0.132 | -0.0512 | 1.069 | 0.996 | -0.0267 | 0.979 |
吸附性能指标 | b 11 | b 22 | b 12 | b 10 | b 20 | b 00 | R 2 |
---|---|---|---|---|---|---|---|
碘值 | 3.287×10-5 | 2.639×10-5 | 5.590×10-5 | 0.895 | 0.903 | 70.001 | 0.992 |
亚甲蓝值 | -0.0011 | -0.0010 | -0.0023 | 1.407 | 1.395 | -37.326 | 0.992 |
丹宁酸值 | 0.0018 | -9.140×10-6 | 0.0015 | 0.932 | 1.038 | -0.138 | 0.997 |
焦糖脱色率 | -0.0109 | 0.132 | -0.0512 | 1.069 | 0.996 | -0.0267 | 0.979 |
吸附性能指标 | 拟合方法 | ||
---|---|---|---|
加权平均 | 线性 | 多项式 | |
碘值 | 0.34 | 0.29 | 0.29 |
亚甲蓝值 | 0.89 | 0.67 | 0.61 |
丹宁酸值 | 3.09 | 3.09 | 2.87 |
焦糖脱色率 | 4.01 | 3.14 | 3.11 |
吸附性能指标 | 拟合方法 | ||
---|---|---|---|
加权平均 | 线性 | 多项式 | |
碘值 | 0.34 | 0.29 | 0.29 |
亚甲蓝值 | 0.89 | 0.67 | 0.61 |
丹宁酸值 | 3.09 | 3.09 | 2.87 |
焦糖脱色率 | 4.01 | 3.14 | 3.11 |
编号 | V t/cm3·g-1 | S BET/m2·g-1 | V mic/cm3·g-1 | V mes/cm3·g-1 | V mes /V t | d a /nm |
---|---|---|---|---|---|---|
DT-830-BCT | 0.596 | 1064 | 0.377 | 0.172 | 0.29 | 2.24 |
DT-830-DCT-1 | 0.465 | 919 | 0.375 | 0.073 | 0.16 | 2.02 |
DT-830-DCT-2 | 0.522 | 952 | 0.364 | 0.103 | 0.20 | 2.19 |
TX-830-ECT | 0.533 | 994 | 0.371 | 0.101 | 0.19 | 2.15 |
XJ-830-BCT | 0.437 | 929 | 0.325 | 0.057 | 0.13 | 1.88 |
XJ-830-DCT | 0.508 | 994 | 0.371 | 0.092 | 0.18 | 2.04 |
DT-830-DCT-3 | 0.577 | 1090 | 0.435 | 0.096 | 0.17 | 2.12 |
DT-1240-BCT-1 | 0.524 | 1028 | 0.366 | 0.112 | 0.21 | 2.04 |
DT-1240-DCT-1 | 0.451 | 898 | 0.367 | 0.068 | 0.15 | 2.01 |
DT-1240-DCT-2 | 0.509 | 923 | 0.377 | 0.106 | 0.21 | 2.21 |
DT-1240-BCT-2 | 0.641 | 939 | 0.371 | 0.266 | 0.41 | 2.73 |
编号 | V t/cm3·g-1 | S BET/m2·g-1 | V mic/cm3·g-1 | V mes/cm3·g-1 | V mes /V t | d a /nm |
---|---|---|---|---|---|---|
DT-830-BCT | 0.596 | 1064 | 0.377 | 0.172 | 0.29 | 2.24 |
DT-830-DCT-1 | 0.465 | 919 | 0.375 | 0.073 | 0.16 | 2.02 |
DT-830-DCT-2 | 0.522 | 952 | 0.364 | 0.103 | 0.20 | 2.19 |
TX-830-ECT | 0.533 | 994 | 0.371 | 0.101 | 0.19 | 2.15 |
XJ-830-BCT | 0.437 | 929 | 0.325 | 0.057 | 0.13 | 1.88 |
XJ-830-DCT | 0.508 | 994 | 0.371 | 0.092 | 0.18 | 2.04 |
DT-830-DCT-3 | 0.577 | 1090 | 0.435 | 0.096 | 0.17 | 2.12 |
DT-1240-BCT-1 | 0.524 | 1028 | 0.366 | 0.112 | 0.21 | 2.04 |
DT-1240-DCT-1 | 0.451 | 898 | 0.367 | 0.068 | 0.15 | 2.01 |
DT-1240-DCT-2 | 0.509 | 923 | 0.377 | 0.106 | 0.21 | 2.21 |
DT-1240-BCT-2 | 0.641 | 939 | 0.371 | 0.266 | 0.41 | 2.73 |
编号 | V t /cm3·g-1 | S BET/m2·g-1 | V mic/cm3·g-1 | V mes/cm3·g-1 | V mes /V t | d a /nm |
---|---|---|---|---|---|---|
AS-1 | 0.529 | 1035 | 0.381 | 0.129 | 0.24 | 2.05 |
AS-2 | 0.495 | 1021 | 0.375 | 0.108 | 0.22 | 1.94 |
AS-3 | 0.454 | 979 | 0.362 | 0.087 | 0.19 | 1.85 |
AS-4 | 0.517 | 993 | 0.385 | 0.102 | 0.20 | 2.08 |
AS-5 | 0.471 | 969 | 0.374 | 0.075 | 0.16 | 1.95 |
AS-6 | 0.542 | 991 | 0.384 | 0.093 | 0.17 | 2.11 |
AS-7 | 0.449 | 930 | 0.364 | 0.078 | 0.17 | 1.93 |
AS-8 | 0.549 | 988 | 0.359 | 0.179 | 0.33 | 2.22 |
编号 | V t /cm3·g-1 | S BET/m2·g-1 | V mic/cm3·g-1 | V mes/cm3·g-1 | V mes /V t | d a /nm |
---|---|---|---|---|---|---|
AS-1 | 0.529 | 1035 | 0.381 | 0.129 | 0.24 | 2.05 |
AS-2 | 0.495 | 1021 | 0.375 | 0.108 | 0.22 | 1.94 |
AS-3 | 0.454 | 979 | 0.362 | 0.087 | 0.19 | 1.85 |
AS-4 | 0.517 | 993 | 0.385 | 0.102 | 0.20 | 2.08 |
AS-5 | 0.471 | 969 | 0.374 | 0.075 | 0.16 | 1.95 |
AS-6 | 0.542 | 991 | 0.384 | 0.093 | 0.17 | 2.11 |
AS-7 | 0.449 | 930 | 0.364 | 0.078 | 0.17 | 1.93 |
AS-8 | 0.549 | 988 | 0.359 | 0.179 | 0.33 | 2.22 |
吸附性能指标 | AS-1 | AS-2 | AS-3 | AS-4 | AS-5 | AS-6 | AS-7 | AS-8 | |
---|---|---|---|---|---|---|---|---|---|
V t | |||||||||
拟合值/cm3?g-1 | 0.548 | 0.516 | 0.485 | 0.504 | 0.499 | 0.515 | 0.473 | 0.583 | |
相对误差/% | 3.59 | 4.24 | 6.83 | 2.51 | 5.94 | 4.98 | 5.34 | 6.19 | |
V mes | |||||||||
拟合值/cm3?g-1 | 0.137 | 0.114 | 0.092 | 0.103 | 0.079 | 0.097 | 0.081 | 0.189 | |
相对误差/% | 6.21 | 5.56 | 5.75 | 0.98 | 5.33 | 4.31 | 3.85 | 5.59 | |
V mic | |||||||||
拟合值/cm3?g-1 | 0.361 | 0.351 | 0.341 | 0.376 | 0.393 | 0.368 | 0.367 | 0.369 | |
相对误差/% | 5.25 | 6.40 | 5.80 | 2.34 | 5.08 | 4.17 | 0.82 | 2.79 | |
S BET | |||||||||
拟合值/m2?g-1 | 1024 | 997 | 970 | 963 | 971 | 973 | 937 | 983 | |
相对误差/% | 1.09 | 2.38 | 0.98 | 3.02 | 0.21 | 1.79 | 0.73 | 0.48 |
吸附性能指标 | AS-1 | AS-2 | AS-3 | AS-4 | AS-5 | AS-6 | AS-7 | AS-8 | |
---|---|---|---|---|---|---|---|---|---|
V t | |||||||||
拟合值/cm3?g-1 | 0.548 | 0.516 | 0.485 | 0.504 | 0.499 | 0.515 | 0.473 | 0.583 | |
相对误差/% | 3.59 | 4.24 | 6.83 | 2.51 | 5.94 | 4.98 | 5.34 | 6.19 | |
V mes | |||||||||
拟合值/cm3?g-1 | 0.137 | 0.114 | 0.092 | 0.103 | 0.079 | 0.097 | 0.081 | 0.189 | |
相对误差/% | 6.21 | 5.56 | 5.75 | 0.98 | 5.33 | 4.31 | 3.85 | 5.59 | |
V mic | |||||||||
拟合值/cm3?g-1 | 0.361 | 0.351 | 0.341 | 0.376 | 0.393 | 0.368 | 0.367 | 0.369 | |
相对误差/% | 5.25 | 6.40 | 5.80 | 2.34 | 5.08 | 4.17 | 0.82 | 2.79 | |
S BET | |||||||||
拟合值/m2?g-1 | 1024 | 997 | 970 | 963 | 971 | 973 | 937 | 983 | |
相对误差/% | 1.09 | 2.38 | 0.98 | 3.02 | 0.21 | 1.79 | 0.73 | 0.48 |
吸附性能指标 | S BET | V t | V mic | V mes | d a |
---|---|---|---|---|---|
碘值 | 0.68 | 0.06 | 0.04 | 0.00 | 0.06 |
亚甲蓝值 | 0.09 | 0.37 | 0.37 | 0.16 | 0.27 |
丹宁酸值 | 0.00 | 0.66 | 0.01 | 0.91 | 0.94 |
焦糖脱色率 | 0.09 | 0.82 | 0.14 | 0.79 | 0.80 |
吸附性能指标 | S BET | V t | V mic | V mes | d a |
---|---|---|---|---|---|
碘值 | 0.68 | 0.06 | 0.04 | 0.00 | 0.06 |
亚甲蓝值 | 0.09 | 0.37 | 0.37 | 0.16 | 0.27 |
丹宁酸值 | 0.00 | 0.66 | 0.01 | 0.91 | 0.94 |
焦糖脱色率 | 0.09 | 0.82 | 0.14 | 0.79 | 0.80 |
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