液相中气泡上升行为与界面传质：实验研究与数值计算

doi:10.16085/j.issn.1000-6613.2017-2641

化工进展 ›› 2019, Vol. 38 ›› Issue (02): 740-751.DOI: 10.16085/j.issn.1000-6613.2017-2641

液相中气泡上升行为与界面传质：实验研究与数值计算

李鑫^1,²(),张攀^2,³,陈光辉^1,²,李建隆^1,²()

1. 青岛科技大学化工学院，山东青岛 266042
2. 山东省多相流体反应与分离工程重点实验室，山东青岛 266042
3. 青岛科技大学机电工程学院，山东青岛 266061

收稿日期:2017-12-21 修回日期:2018-01-26 出版日期:2019-02-05 发布日期:2019-02-05
通讯作者: 李建隆
作者简介:<named-content content-type="corresp-name">李鑫</named-content>（1992—），男，博士研究生，研究方向为传质与分离工程。E-mail：<email>qdlx2015@126.com</email>。|李建隆，教授，博士生导师，研究方向为多相流体的流动与分离。E-mail：<email>ljlong@qust.edu.cn</email>。
基金资助:
山东省高等学校科技计划一般项目A类(J17KA107);青岛市科技成果转化计划-科技惠民专项(16-6-2-50-nsh)

Rising behavior of bubbles and interfacial mass transfer in liquid: experimental study and numerical simulation

Xin LI^1,²(),Pan ZHANG^2,³,Guanghui CHEN^1,²,Jianlong LI^1,²()

1. College of Chemical Engineering, Qingdao University of Science and Technology, Qingdao 266042, Shandong, China
2. Shandong Key Laboratory of Multi-phase Fluid Reaction Engineering and Separation Engineering, Qingdao 266042, Shandong, China
3. College of Electromechanical Engineering, Qingdao University of Science and Technology, Qingdao 266061, Shandong, China

Received:2017-12-21 Revised:2018-01-26 Online:2019-02-05 Published:2019-02-05
Contact: Jianlong LI

摘要/Abstract

摘要：

在工业生产过程中，气泡在液相中的上升行为及气液界面的传质行为极为常见。本文针对不同条件下气泡上升过程的实验研究方法以及数值计算方法进行了总结。从实验与数值计算的角度，综述了单气泡上升过程的影响因素、多气泡上升过程聚并与破裂的现象和机理以及工业装置中气液两相流型和气泡特性，并对传质模型进行了归纳，主要关注了气侧-界面传质模型的研究现状。综述结果表明：当前对于单气泡上升行为的研究较为充分，而对于多气泡的行为机理的研究尚需深入。此外，受到研究手段的限制，进行气侧-界面传质模型研究具有一定挑战性。针对当前的相关研究进展和存在的问题，对今后气泡上升行为和传质行为的研究提出以下建议，即开展气泡聚并与破裂可控性研究，强化对气侧-界面传质过程的研究，包括泡内流体行为可视化研究和相关传质模型的建立。

关键词: 气泡, 上升行为, 传质, 多相流, 模型

Abstract:

In the industrial processes, rising behavior of bubbles in the liquid and mass transfer on the gas-liquid interface are very common. In this paper, experimental methods and numerical simulation methods are summarized under different conditions. In terms of experiments and numerical simulations, impact factors of single bubble rising behavior, phenomenon and mechanism of coalescence and break up for multiple bubbles, bubble flow pattern and properties in industrial devices, and mass transfer model, especially for gas-interface mass transfer model, are summed up. The results show that the studies about single bubble behavior are sufficient while for the multiple bubbles, more works need to be done. Besides, it is challenging to establish gas-interface mass transfer model due to the limit of research tools. According to the relative research progress and problems, the following suggestions about the future research directions conducting controllability study of coalescence and break up for bubbles, and strengthening of research on gas-interface mass transfer including the research of visualization of the internal flow and convective mass transfer in bubbles.

Key words: bubble, rising behavior, mass transfer, multiphase flow, model

中图分类号:

TQ021.4

李鑫, 张攀, 陈光辉, 李建隆. 液相中气泡上升行为与界面传质：实验研究与数值计算[J]. 化工进展, 2019, 38(02): 740-751.

Xin LI, Pan ZHANG, Guanghui CHEN, Jianlong LI. Rising behavior of bubbles and interfacial mass transfer in liquid: experimental study and numerical simulation[J]. Chemical Industry and Engineering Progress, 2019, 38(02): 740-751.

图/表 6

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多相流数值计算模型	优点	缺点
边界积分法^[25]	计算量小，能准确模拟表面张力效应	难以模拟流场的拓扑变化和黏性效应
界面追踪法^[26]	计算精确度较高	处理拓扑几何变化计算量大
水平集方法^[27]	模拟相界面动态行为效果较好	处理三维数值模拟效果不理想
流体体积函数模型	利用几何重构实现界面追踪，可清晰地区分各相主体以及界面	计算光滑几何特性精确度偏低
水平集-流体体积函数耦合法^[28]	模拟界面及流场变化效果较好	计算过程复杂，计算量较大
混合模型^[29]	可模拟各相速度不同的多相流以及强烈耦合的各向同性多相流	对界面特性的计算结果不理想
欧拉模型	计算精确度较高，适用范围广	由于各相采用不同动量方程描述，导致计算量很大

多相流数值计算模型	优点	缺点
边界积分法^[25]	计算量小，能准确模拟表面张力效应	难以模拟流场的拓扑变化和黏性效应
界面追踪法^[26]	计算精确度较高	处理拓扑几何变化计算量大
水平集方法^[27]	模拟相界面动态行为效果较好	处理三维数值模拟效果不理想
流体体积函数模型	利用几何重构实现界面追踪，可清晰地区分各相主体以及界面	计算光滑几何特性精确度偏低
水平集-流体体积函数耦合法^[28]	模拟界面及流场变化效果较好	计算过程复杂，计算量较大
混合模型^[29]	可模拟各相速度不同的多相流以及强烈耦合的各向同性多相流	对界面特性的计算结果不理想
欧拉模型	计算精确度较高，适用范围广	由于各相采用不同动量方程描述，导致计算量很大

气液体系	多相流模型	气泡类型	作者及发表年份
空气-水	VOF	多气泡	王乐等^[30], 2016
空气-水	VOF	多气泡	Zhang等^[31], 2012
空气-水	VOF	多气泡	Akhtar等^[32], 2007
空气-水	VOF	单气泡	程军明等^[33], 2014
空气-水	VOF	单气泡	Guan等^[34], 2014
空气-水	VOF	单气泡	蔡杰进等^[35], 2013
空气-水	VOF	单气泡	赵婷婷等^[36], 2013
空气-水	VOF	单气泡	徐玲君等^[37], 2012
空气-水	VOF	单气泡	Goel等^[38], 2009
空气-水	Eulerian	多气泡	Pourtousi等^[39], 2015
空气-水	Eulerian	多气泡	Rampure等^[40], 2007
空气-水	Eulerian	多气泡	Chen等^[41], 2005
空气-水	Eulerian	多气泡	Sanyal等^[42], 1999
空气-水	Eulerian	单气泡	鞠花等^[43], 2011
空气-羧甲基纤维素钠溶液	VOF	单气泡	Premlata等^[44], 2017
空气-0.4%羧甲基纤维素钠溶液	VOF	多气泡	Liu等^[45], 2014
空气-0.5%羧甲基纤维素钠溶液	VOF	多气泡	Liu等^[46], 2013
空气-甘油+水	VOF-IB	单气泡/多气泡	Baltussen等^[47], 2017
空气-水/甘油+水	VOF	单气泡	Rabha等^[48], 2010
氮气-离子液体	VOF	单气泡	Wang等^[49], 2010
空气-液态流体（未公开）	VOF	单气泡	Taha等^[50], 2004

气液体系	多相流模型	气泡类型	作者及发表年份
空气-水	VOF	多气泡	王乐等^[30], 2016
空气-水	VOF	多气泡	Zhang等^[31], 2012
空气-水	VOF	多气泡	Akhtar等^[32], 2007
空气-水	VOF	单气泡	程军明等^[33], 2014
空气-水	VOF	单气泡	Guan等^[34], 2014
空气-水	VOF	单气泡	蔡杰进等^[35], 2013
空气-水	VOF	单气泡	赵婷婷等^[36], 2013
空气-水	VOF	单气泡	徐玲君等^[37], 2012
空气-水	VOF	单气泡	Goel等^[38], 2009
空气-水	Eulerian	多气泡	Pourtousi等^[39], 2015
空气-水	Eulerian	多气泡	Rampure等^[40], 2007
空气-水	Eulerian	多气泡	Chen等^[41], 2005
空气-水	Eulerian	多气泡	Sanyal等^[42], 1999
空气-水	Eulerian	单气泡	鞠花等^[43], 2011
空气-羧甲基纤维素钠溶液	VOF	单气泡	Premlata等^[44], 2017
空气-0.4%羧甲基纤维素钠溶液	VOF	多气泡	Liu等^[45], 2014
空气-0.5%羧甲基纤维素钠溶液	VOF	多气泡	Liu等^[46], 2013
空气-甘油+水	VOF-IB	单气泡/多气泡	Baltussen等^[47], 2017
空气-水/甘油+水	VOF	单气泡	Rabha等^[48], 2010
氮气-离子液体	VOF	单气泡	Wang等^[49], 2010
空气-液态流体（未公开）	VOF	单气泡	Taha等^[50], 2004

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液相中气泡上升行为与界面传质：实验研究与数值计算

Rising behavior of bubbles and interfacial mass transfer in liquid: experimental study and numerical simulation

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