Chemical Industry and Engineering Progress ›› 2023, Vol. 42 ›› Issue (11): 5831-5841.DOI: 10.16085/j.issn.1000-6613.2023-0010
• Materials science and technology • Previous Articles
CAO Mingmin(), HAN Chengle, YANG Fang, CHEN Yuhuan()
Received:
2023-01-04
Revised:
2023-02-24
Online:
2023-12-15
Published:
2023-11-20
Contact:
CHEN Yuhuan
通讯作者:
陈玉焕
作者简介:
曹明敏(1997—),女,硕士研究生,研究方向为绿色功能材料。E-mail:986628549@qq.com。
CLC Number:
CAO Mingmin, HAN Chengle, YANG Fang, CHEN Yuhuan. CO2 capture and separation by ionic liquid-metal organic framework composite materials[J]. Chemical Industry and Engineering Progress, 2023, 42(11): 5831-5841.
曹明敏, 韩铖乐, 杨芳, 陈玉焕. 离子液体/金属有机框架复合材料捕集分离CO2[J]. 化工进展, 2023, 42(11): 5831-5841.
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体系 | 吸附量 | 理想选择性α | 文献 | ||||||
---|---|---|---|---|---|---|---|---|---|
ILs | MOFs | CO2/N2 | CO2/CH4 | ||||||
MOFs@ILs | 30%(质量分数)[BMIm][MeSO3] | ZIF-8 | 约12.5mL(STP)/g | 约1.5 | 约2 | [ | |||
30%(质量分数)[BMIm][CF3SO3] | ZIF-8 | 约11.8mL(STP)/g | 约0.7 | 约3 | [ | ||||
30%(质量分数)[BMIm][MeSO4] | ZIF-8 | 约12.7mL(STP)/g | 约3.3 | 约1.8 | [ | ||||
30%(质量分数)[BMIm][OCSO4] | ZIF-8 | 约5.5mL(STP)/g | 约0.6 | 约1.4 | [ | ||||
5%(质量分数)[BMIm][AC] | HKUST-1 | 4.4mmol/g | [ | ||||||
10%(质量分数)[BMIm][AC] | HKUST-1 | 2.9mmol/g | [ | ||||||
20%(质量分数)[BMIm][AC] | HKUST-1 | 1.9mmol/g | [ | ||||||
3.44%(质量分数)[BMIm][BF4] | UiO-66 | 约32cm3/g | 8.1 | [ | |||||
7.8%(质量分数)[BMIm][BF4] | ZIF-8 | 约12cm3/g | 7.5 | [ | |||||
2.38%(质量分数)[BMIm][BF4] | CuBTC | 约8cm3/g | 15.3 | [ | |||||
30%(质量分数)[EMIm][DEP] | CuBTC | 约44mL/g | 7.4 | [ | |||||
30%(质量分数)[BMIm][SCN] | ZIF-8 | 约6.5mL/g | 约11 | 约5 | [ | ||||
5%(质量分数)[BMIm][BF4] | ZIF-8 | 约250mL/g | 15.81 | 5.57 | [ | ||||
9.3%(摩尔分数)[BMIm]2[CoCl4] | ZIF-8 | 0.43mmol/g | 7.5 | 2.7 | [ | ||||
9.3%(摩尔分数)[BMIm]2[NiCl4] | ZIF-8 | 0.40mmol/g | 7.5 | 2.7 | [ | ||||
9.3%(摩尔分数)[BMIm]2[FeCl4] | ZIF-8 | 0.41mmol/g | 7.1 | 2.8 | [ | ||||
9.3%(摩尔分数)[BMIm]2[Co(NCS)4] | ZIF-8 | 0.30mmol/g | 6.4 | 2.4 | [ | ||||
9.3%(摩尔分数)[BMIm]2[MnCl4] | ZIF-8 | 0.32mmol/g | 7.9 | 3.3 | [ | ||||
50%(质量分数)[EMIm][DCN] | MIL-101(Al) | 约3.2mmol/g | [ | ||||||
PIL | MIL-101(Cr) | 62cm3/g | [ | ||||||
20%(质量分数)[BMIm][BF4] | ZIF-8 | 10.5mL(STP)/g | 约8 | 约3 | [ | ||||
IL@MOFs | [C2OHMIM][DCA] | ZIF-8 | 3mL(STP)/g | 11 | [ | ||||
[HemIm][DCA] | ZIF-8 | 8.6cm3/g | 30 | [ | |||||
IL@MOFs@IL | [TETA]L | ZIF-8 | 1.53mmol/g | 1688① | 260② | [ | |||
IL-MOFs | [PMIm][SO3]-NaCl | UiO-67 | 47.9cm3/g | 44.21② | [ | ||||
[NAIm]Br | ZIF-67 | 24.8cm3/g | [ | ||||||
PIL-NH2 | Cu3(BTC)2 | 19.5cm3/g | [ |
体系 | 吸附量 | 理想选择性α | 文献 | ||||||
---|---|---|---|---|---|---|---|---|---|
ILs | MOFs | CO2/N2 | CO2/CH4 | ||||||
MOFs@ILs | 30%(质量分数)[BMIm][MeSO3] | ZIF-8 | 约12.5mL(STP)/g | 约1.5 | 约2 | [ | |||
30%(质量分数)[BMIm][CF3SO3] | ZIF-8 | 约11.8mL(STP)/g | 约0.7 | 约3 | [ | ||||
30%(质量分数)[BMIm][MeSO4] | ZIF-8 | 约12.7mL(STP)/g | 约3.3 | 约1.8 | [ | ||||
30%(质量分数)[BMIm][OCSO4] | ZIF-8 | 约5.5mL(STP)/g | 约0.6 | 约1.4 | [ | ||||
5%(质量分数)[BMIm][AC] | HKUST-1 | 4.4mmol/g | [ | ||||||
10%(质量分数)[BMIm][AC] | HKUST-1 | 2.9mmol/g | [ | ||||||
20%(质量分数)[BMIm][AC] | HKUST-1 | 1.9mmol/g | [ | ||||||
3.44%(质量分数)[BMIm][BF4] | UiO-66 | 约32cm3/g | 8.1 | [ | |||||
7.8%(质量分数)[BMIm][BF4] | ZIF-8 | 约12cm3/g | 7.5 | [ | |||||
2.38%(质量分数)[BMIm][BF4] | CuBTC | 约8cm3/g | 15.3 | [ | |||||
30%(质量分数)[EMIm][DEP] | CuBTC | 约44mL/g | 7.4 | [ | |||||
30%(质量分数)[BMIm][SCN] | ZIF-8 | 约6.5mL/g | 约11 | 约5 | [ | ||||
5%(质量分数)[BMIm][BF4] | ZIF-8 | 约250mL/g | 15.81 | 5.57 | [ | ||||
9.3%(摩尔分数)[BMIm]2[CoCl4] | ZIF-8 | 0.43mmol/g | 7.5 | 2.7 | [ | ||||
9.3%(摩尔分数)[BMIm]2[NiCl4] | ZIF-8 | 0.40mmol/g | 7.5 | 2.7 | [ | ||||
9.3%(摩尔分数)[BMIm]2[FeCl4] | ZIF-8 | 0.41mmol/g | 7.1 | 2.8 | [ | ||||
9.3%(摩尔分数)[BMIm]2[Co(NCS)4] | ZIF-8 | 0.30mmol/g | 6.4 | 2.4 | [ | ||||
9.3%(摩尔分数)[BMIm]2[MnCl4] | ZIF-8 | 0.32mmol/g | 7.9 | 3.3 | [ | ||||
50%(质量分数)[EMIm][DCN] | MIL-101(Al) | 约3.2mmol/g | [ | ||||||
PIL | MIL-101(Cr) | 62cm3/g | [ | ||||||
20%(质量分数)[BMIm][BF4] | ZIF-8 | 10.5mL(STP)/g | 约8 | 约3 | [ | ||||
IL@MOFs | [C2OHMIM][DCA] | ZIF-8 | 3mL(STP)/g | 11 | [ | ||||
[HemIm][DCA] | ZIF-8 | 8.6cm3/g | 30 | [ | |||||
IL@MOFs@IL | [TETA]L | ZIF-8 | 1.53mmol/g | 1688① | 260② | [ | |||
IL-MOFs | [PMIm][SO3]-NaCl | UiO-67 | 47.9cm3/g | 44.21② | [ | ||||
[NAIm]Br | ZIF-67 | 24.8cm3/g | [ | ||||||
PIL-NH2 | Cu3(BTC)2 | 19.5cm3/g | [ |
填料 | 聚合物基质 | 填料质量分数 /% | 操作条件 | 渗透率 /bar | 选择性 | 文献 | ||
---|---|---|---|---|---|---|---|---|
T/K | Δp/bar | CO2/N2 | CO2/CH4 | |||||
6%(体积分数)[BMIm][Tf2N]/ZIF-8 | PSF | 303 | 6 | 约312 | 100 | 41 | [ | |
2%(质量分数)[EMIm][C(CN)3]/Mg-MOF-74 | Matrimid®5218 | 2 | 303 | 0.7 | 36.13 | [ | ||
2%(质量分数)TMGA/MOF-5 | Matrimid®5218 | 2 | 303 | 0.7 | 35.48 | [ | ||
8%(质量分数)[BMIm][PF6]/ZIF-8 | Pebax | 25 | 298 | 2 | 117 | 84.5 | [ | |
50%(质量分数)[C3NH2BIm][Tf2N]/NH2-MIL-101(Cr) | PIM-1 | 5 | 298 | 3 | 2979 | 37.24 | [ | |
67%(质量分数)[EMIm][Tf2N]/HKUST-1 | 6FDA-Durene Polyimide | 30 | 298 | 1.985 | 1101.6 | 27.1 | 29.3 | [ |
83%(质量分数)[BMIm][Tf2N]/UiO-66-NH2 | PIM-1 | 10 | 293 | 1 | 8283.4 | 12.3 | 22.5 | [ |
5%(质量分数)[BMIm][BF4]/ZIF-67 | 6FDA-Durene Polyimide | 10 | 298 | 2 | 779.01 | 18.48 | 18.76 | [ |
5%(质量分数)[BMIm][BF4]/ZIF-67 | 6FDA-Durene Polyimide | 20 | 298 | 2 | 1254.64 | 25.70 | 24.00 | [ |
5%(质量分数)[EMIm][Tf2N]/ZIF-67 | 6FDA-Durene Polyimide | 10 | 298 | 2 | 1030.9 | 20.87 | 19.40 | [ |
5%(质量分数)[EMIm][Tf2N]/ZIF-67 | 6FDA-Durene Polyimide | 20 | 298 | 2 | 1426 | 25.28 | 25.49 | [ |
5%(质量分数)[BMIm][Tf2N]/ZIF-67 | 6FDA-Durene Polyimide | 10 | 298 | 2 | 672 | 23.54 | 22.77 | [ |
5%(质量分数)[BMIm][Tf2N]/ZIF-67 | 6FDA-Durene/(P) | 20 | 298 | 2 | 889 | 28.09 | 28.05 | [ |
[EMIm][Tf2N]/ZIF-8 | P[VBIm][Tf2N] | 25.8 | 308 | 3.5 | 1062.4 | 24.2 | 12.34 | [ |
[BMIm][BF4]/Zr-Fc MOF | Polycarbonate | 293 | 0.49 | 66.8 | 216.9 | 41.7 | [ |
填料 | 聚合物基质 | 填料质量分数 /% | 操作条件 | 渗透率 /bar | 选择性 | 文献 | ||
---|---|---|---|---|---|---|---|---|
T/K | Δp/bar | CO2/N2 | CO2/CH4 | |||||
6%(体积分数)[BMIm][Tf2N]/ZIF-8 | PSF | 303 | 6 | 约312 | 100 | 41 | [ | |
2%(质量分数)[EMIm][C(CN)3]/Mg-MOF-74 | Matrimid®5218 | 2 | 303 | 0.7 | 36.13 | [ | ||
2%(质量分数)TMGA/MOF-5 | Matrimid®5218 | 2 | 303 | 0.7 | 35.48 | [ | ||
8%(质量分数)[BMIm][PF6]/ZIF-8 | Pebax | 25 | 298 | 2 | 117 | 84.5 | [ | |
50%(质量分数)[C3NH2BIm][Tf2N]/NH2-MIL-101(Cr) | PIM-1 | 5 | 298 | 3 | 2979 | 37.24 | [ | |
67%(质量分数)[EMIm][Tf2N]/HKUST-1 | 6FDA-Durene Polyimide | 30 | 298 | 1.985 | 1101.6 | 27.1 | 29.3 | [ |
83%(质量分数)[BMIm][Tf2N]/UiO-66-NH2 | PIM-1 | 10 | 293 | 1 | 8283.4 | 12.3 | 22.5 | [ |
5%(质量分数)[BMIm][BF4]/ZIF-67 | 6FDA-Durene Polyimide | 10 | 298 | 2 | 779.01 | 18.48 | 18.76 | [ |
5%(质量分数)[BMIm][BF4]/ZIF-67 | 6FDA-Durene Polyimide | 20 | 298 | 2 | 1254.64 | 25.70 | 24.00 | [ |
5%(质量分数)[EMIm][Tf2N]/ZIF-67 | 6FDA-Durene Polyimide | 10 | 298 | 2 | 1030.9 | 20.87 | 19.40 | [ |
5%(质量分数)[EMIm][Tf2N]/ZIF-67 | 6FDA-Durene Polyimide | 20 | 298 | 2 | 1426 | 25.28 | 25.49 | [ |
5%(质量分数)[BMIm][Tf2N]/ZIF-67 | 6FDA-Durene Polyimide | 10 | 298 | 2 | 672 | 23.54 | 22.77 | [ |
5%(质量分数)[BMIm][Tf2N]/ZIF-67 | 6FDA-Durene/(P) | 20 | 298 | 2 | 889 | 28.09 | 28.05 | [ |
[EMIm][Tf2N]/ZIF-8 | P[VBIm][Tf2N] | 25.8 | 308 | 3.5 | 1062.4 | 24.2 | 12.34 | [ |
[BMIm][BF4]/Zr-Fc MOF | Polycarbonate | 293 | 0.49 | 66.8 | 216.9 | 41.7 | [ |
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