Chemical Industry and Engineering Progress ›› 2022, Vol. 41 ›› Issue (10): 5669-5676.DOI: 10.16085/j.issn.1000-6613.2022-0015
• Resources and environmental engineering • Previous Articles Next Articles
WANG Dongliang1,2(), XIE Jiangpeng1,2, MENG Wenliang1,2, LI Jingwei1,2, ZHOU Huairong1,2()
Received:
2022-01-04
Revised:
2022-06-06
Online:
2022-10-21
Published:
2022-10-20
Contact:
ZHOU Huairong
王东亮1,2(), 谢江鹏1,2, 孟文亮1,2, 李婧玮1,2, 周怀荣1,2()
通讯作者:
周怀荣
作者简介:
王东亮(1982—),男,博士,副教授,研究方向为化工过程集成与资源综合利用。E-mail:wangdl@lut.edu.cn。
基金资助:
CLC Number:
WANG Dongliang, XIE Jiangpeng, MENG Wenliang, LI Jingwei, ZHOU Huairong. Multi-objective capacity and heat analysis of amine-based SO2 capture process from acidity coefficient (pKa) model[J]. Chemical Industry and Engineering Progress, 2022, 41(10): 5669-5676.
王东亮, 谢江鹏, 孟文亮, 李婧玮, 周怀荣. 基于酸度系数(pKa)模型的胺法SO2捕集过程多目标效能分析[J]. 化工进展, 2022, 41(10): 5669-5676.
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类别 | A | B | C | D | 温度区间/K | 参考 |
---|---|---|---|---|---|---|
lnKs1(SO2) | -10.9670 | 1972.5 | — | — | — | Rabe等[ |
lnKs1(HSO | -357.5700 | 5477.1 | 65.31 | -0.1624 | — | Millero等[ |
lnK(H2SO4) | >10 | — | — | — | — | Sippola等[ |
lnK(HSO | -49.7086 | 178.1142 | 10.9523 | -0.0598 | — | Sippola等[ |
lnK(EDAH+) | -79.7113 | -6508.6363 | 14.4126 | -0.0169 | 298.15~398.15 | 拟合 |
lnK(PZH+) | -62.6234 | -7025.0400 | 11.8682 | -0.0136 | 298.15~398.15 | 拟合 |
lnK(HEPH+) | -69.6302 | -6496.8100 | 13.1533 | -0.0154 | 298.15~398.15 | 拟合 |
lnK(DIHEPH+) | -56.7455 | -5761.7300 | 10.7373 | -0.0123 | 298.15~398.15 | 拟合 |
lnK(HEHPPH+) | -75.0596 | -6708.4600 | 14.0755 | -0.0172 | 298.15~398.15 | 拟合 |
lnK(EDAH | -66.4837 | -5110.9300 | 12.7213 | -0.0140 | 298.15~398.15 | 拟合 |
lnK(PZH | -92.5319 | -3609.9200 | 17.2128 | -0.0208 | 298.15~398.15 | 拟合 |
lnK(HEPH | -84.1281 | -2928.1100 | 15.6410 | -0.0190 | 298.15~398.15 | 拟合 |
lnK(DIHEPH | -87.4632 | -2832.4700 | 16.4588 | -0.0199 | 298.15~398.15 | 拟合 |
lnK(HEHPPH | -66.4512 | -3557.3000 | 12.5968 | -0.0142 | 298.15~398.15 | 拟合 |
类别 | A | B | C | D | 温度区间/K | 参考 |
---|---|---|---|---|---|---|
lnKs1(SO2) | -10.9670 | 1972.5 | — | — | — | Rabe等[ |
lnKs1(HSO | -357.5700 | 5477.1 | 65.31 | -0.1624 | — | Millero等[ |
lnK(H2SO4) | >10 | — | — | — | — | Sippola等[ |
lnK(HSO | -49.7086 | 178.1142 | 10.9523 | -0.0598 | — | Sippola等[ |
lnK(EDAH+) | -79.7113 | -6508.6363 | 14.4126 | -0.0169 | 298.15~398.15 | 拟合 |
lnK(PZH+) | -62.6234 | -7025.0400 | 11.8682 | -0.0136 | 298.15~398.15 | 拟合 |
lnK(HEPH+) | -69.6302 | -6496.8100 | 13.1533 | -0.0154 | 298.15~398.15 | 拟合 |
lnK(DIHEPH+) | -56.7455 | -5761.7300 | 10.7373 | -0.0123 | 298.15~398.15 | 拟合 |
lnK(HEHPPH+) | -75.0596 | -6708.4600 | 14.0755 | -0.0172 | 298.15~398.15 | 拟合 |
lnK(EDAH | -66.4837 | -5110.9300 | 12.7213 | -0.0140 | 298.15~398.15 | 拟合 |
lnK(PZH | -92.5319 | -3609.9200 | 17.2128 | -0.0208 | 298.15~398.15 | 拟合 |
lnK(HEPH | -84.1281 | -2928.1100 | 15.6410 | -0.0190 | 298.15~398.15 | 拟合 |
lnK(DIHEPH | -87.4632 | -2832.4700 | 16.4588 | -0.0199 | 298.15~398.15 | 拟合 |
lnK(HEHPPH | -66.4512 | -3557.3000 | 12.5968 | -0.0142 | 298.15~398.15 | 拟合 |
温度T/K | 解离自由能ΔG1/kJ·mol-1 | 解离自由能∆G2/kJ·mol-1 | |||||||||
---|---|---|---|---|---|---|---|---|---|---|---|
EDAH+ | PZH+ | HEPH+ | DIHEPH+ | HEHPPH+ | EDAH | PZH | HEPH | DIHEPH | HEHPPH | ||
298.15 | 55.6187 | 55.9831 | 52.2001 | 45.973 | 47.1383 | 37.9241 | 31.6248 | 25.9967 | 22.6101 | 23.8055 | |
308.15 | 54.628 | 54.9944 | 51.1718 | 45.0618 | 46.1351 | 36.8039 | 30.5023 | 24.9643 | 21.4439 | 22.7563 | |
318.15 | 53.3262 | 53.6688 | 49.7306 | 43.657 | 44.6075 | 35.9446 | 29.6664 | 24.2946 | 20.7295 | 22.1856 | |
328.15 | 52.5966 | 52.9567 | 49.0525 | 43.1891 | 44.066 | 34.4923 | 28.1971 | 22.8366 | 19.0488 | 20.612 | |
338.15 | 51.5683 | 51.9323 | 47.9866 | 42.2486 | 43.0294 | 33.3303 | 27.0363 | 21.7666 | 17.8491 | 19.5294 | |
348.15 | 50.5358 | 50.904 | 46.9165 | 41.2998 | 41.9844 | 32.1641 | 25.8701 | 20.6923 | 16.6369 | 18.4426 | |
358.15 | 49.495 | 49.8674 | 45.8381 | 40.3467 | 40.931 | 30.9853 | 24.6913 | 19.6097 | 15.4205 | 17.3474 | |
368.15 | 48.4542 | 48.8224 | 44.7597 | 39.3895 | 39.8819 | 29.8024 | 23.5126 | 18.5187 | 14.2 | 16.2439 | |
378.15 | 47.405 | 47.7816 | 43.6729 | 38.4323 | 38.8243 | 28.6152 | 22.3255 | 17.4319 | 12.9711 | 15.1404 | |
388.15 | 46.3475 | 46.7282 | 42.5777 | 37.4625 | 37.7584 | 27.4156 | 21.1342 | 16.3367 | 11.738 | 14.0285 | |
398.15 | 45.2899 | 45.6707 | 41.4825 | 36.4928 | 36.6967 | 26.2159 | 19.9429 | 15.2332 | 10.5049 | 12.9124 |
温度T/K | 解离自由能ΔG1/kJ·mol-1 | 解离自由能∆G2/kJ·mol-1 | |||||||||
---|---|---|---|---|---|---|---|---|---|---|---|
EDAH+ | PZH+ | HEPH+ | DIHEPH+ | HEHPPH+ | EDAH | PZH | HEPH | DIHEPH | HEHPPH | ||
298.15 | 55.6187 | 55.9831 | 52.2001 | 45.973 | 47.1383 | 37.9241 | 31.6248 | 25.9967 | 22.6101 | 23.8055 | |
308.15 | 54.628 | 54.9944 | 51.1718 | 45.0618 | 46.1351 | 36.8039 | 30.5023 | 24.9643 | 21.4439 | 22.7563 | |
318.15 | 53.3262 | 53.6688 | 49.7306 | 43.657 | 44.6075 | 35.9446 | 29.6664 | 24.2946 | 20.7295 | 22.1856 | |
328.15 | 52.5966 | 52.9567 | 49.0525 | 43.1891 | 44.066 | 34.4923 | 28.1971 | 22.8366 | 19.0488 | 20.612 | |
338.15 | 51.5683 | 51.9323 | 47.9866 | 42.2486 | 43.0294 | 33.3303 | 27.0363 | 21.7666 | 17.8491 | 19.5294 | |
348.15 | 50.5358 | 50.904 | 46.9165 | 41.2998 | 41.9844 | 32.1641 | 25.8701 | 20.6923 | 16.6369 | 18.4426 | |
358.15 | 49.495 | 49.8674 | 45.8381 | 40.3467 | 40.931 | 30.9853 | 24.6913 | 19.6097 | 15.4205 | 17.3474 | |
368.15 | 48.4542 | 48.8224 | 44.7597 | 39.3895 | 39.8819 | 29.8024 | 23.5126 | 18.5187 | 14.2 | 16.2439 | |
378.15 | 47.405 | 47.7816 | 43.6729 | 38.4323 | 38.8243 | 28.6152 | 22.3255 | 17.4319 | 12.9711 | 15.1404 | |
388.15 | 46.3475 | 46.7282 | 42.5777 | 37.4625 | 37.7584 | 27.4156 | 21.1342 | 16.3367 | 11.738 | 14.0285 | |
398.15 | 45.2899 | 45.6707 | 41.4825 | 36.4928 | 36.6967 | 26.2159 | 19.9429 | 15.2332 | 10.5049 | 12.9124 |
SO2分压p(SO2) /Pa | 浓度 | 相对误差 /% | |||
---|---|---|---|---|---|
c(EDA) /mol·L-1 | c(H3PO4) /mol·L-1 | cs(exp) /mol·L-1 | cs(cal) /mol·L-1 | ||
143 | 0.3 | 0 | 0.5610 | 0.5945 | -5.6350 |
204 | 0.3 | 0 | 0.5630 | 0.5970 | -5.6951 |
294 | 0.3 | 0 | 0.5820 | 0.5992 | -2.8705 |
112 | 0.3 | 0.13 | 0.4820 | 0.4653 | 3.5891 |
232 | 0.3 | 0.13 | 0.4660 | 0.4700 | -0.8511 |
301 | 0.3 | 0.13 | 0.4680 | 0.4715 | -0.7423 |
108 | 0.3 | 0.26 | 0.3325 | 0.3380 | -1.6272 |
298 | 0.3 | 0.26 | 0.3450 | 0.3444 | 0.1742 |
373 | 0.3 | 0.26 | 0.3525 | 0.3462 | 1.8198 |
118 | 0.3 | 0.39 | 0.2235 | 0.2122 | 5.3252 |
252 | 0.3 | 0.39 | 0.2288 | 0.2180 | 4.9541 |
337 | 0.3 | 0.39 | 0.2341 | 0.2211 | 5.8797 |
SO2分压p(SO2) /Pa | 浓度 | 相对误差 /% | |||
---|---|---|---|---|---|
c(EDA) /mol·L-1 | c(H3PO4) /mol·L-1 | cs(exp) /mol·L-1 | cs(cal) /mol·L-1 | ||
143 | 0.3 | 0 | 0.5610 | 0.5945 | -5.6350 |
204 | 0.3 | 0 | 0.5630 | 0.5970 | -5.6951 |
294 | 0.3 | 0 | 0.5820 | 0.5992 | -2.8705 |
112 | 0.3 | 0.13 | 0.4820 | 0.4653 | 3.5891 |
232 | 0.3 | 0.13 | 0.4660 | 0.4700 | -0.8511 |
301 | 0.3 | 0.13 | 0.4680 | 0.4715 | -0.7423 |
108 | 0.3 | 0.26 | 0.3325 | 0.3380 | -1.6272 |
298 | 0.3 | 0.26 | 0.3450 | 0.3444 | 0.1742 |
373 | 0.3 | 0.26 | 0.3525 | 0.3462 | 1.8198 |
118 | 0.3 | 0.39 | 0.2235 | 0.2122 | 5.3252 |
252 | 0.3 | 0.39 | 0.2288 | 0.2180 | 4.9541 |
337 | 0.3 | 0.39 | 0.2341 | 0.2211 | 5.8797 |
有机胺 | a | b | c | d |
---|---|---|---|---|
EDA | -14.2062 | 21.6396 | -10.8574 | 83.3219 |
PZ | -8.1086 | 11.8772 | -6.9219 | 76.1474 |
HEP | -23.8924 | 25.9303 | -10.7243 | 67.6164 |
DIHEP | -91.1772 | 66.9002 | -18.0294 | 68.1945 |
HEHPP | -19.6444 | 24.5696 | -11.1515 | 68.9849 |
有机胺 | a | b | c | d |
---|---|---|---|---|
EDA | -14.2062 | 21.6396 | -10.8574 | 83.3219 |
PZ | -8.1086 | 11.8772 | -6.9219 | 76.1474 |
HEP | -23.8924 | 25.9303 | -10.7243 | 67.6164 |
DIHEP | -91.1772 | 66.9002 | -18.0294 | 68.1945 |
HEHPP | -19.6444 | 24.5696 | -11.1515 | 68.9849 |
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