Chemical Industry and Engineering Progress ›› 2022, Vol. 41 ›› Issue (12): 6395-6407.DOI: 10.16085/j.issn.1000-6613.2022-0404
• Materials science and technology • Previous Articles Next Articles
GAO Yifei1,2(), YI Qun3, QI Kai1,2(), GAO Lili1,2(), LI Xuelian1,2
Received:
2022-03-16
Revised:
2022-04-14
Online:
2022-12-29
Published:
2022-12-20
Contact:
QI Kai, GAO Lili
高逸飞1,2(), 易群3, 齐凯1,2(), 高丽丽1,2(), 李雪莲1,2
通讯作者:
齐凯,高丽丽
作者简介:
高逸飞(1998—),男,硕士研究生,研究方向为气体分离纯化材料开发与设计。E-mail:1197182162@qq.com。
基金资助:
CLC Number:
GAO Yifei, YI Qun, QI Kai, GAO Lili, LI Xuelian. Research status and application in H2/CH4 separation of MOFs-based membrane[J]. Chemical Industry and Engineering Progress, 2022, 41(12): 6395-6407.
高逸飞, 易群, 齐凯, 高丽丽, 李雪莲. MOFs基膜材料的研究现状及其在H2/CH4分离中的应用[J]. 化工进展, 2022, 41(12): 6395-6407.
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URL: https://hgjz.cip.com.cn/EN/10.16085/j.issn.1000-6613.2022-0404
分离材料 | 孔径/Å | 设计原理 | 制备方法 | 分离条件/℃ | H2/CH4选择性 | H2通量/mol·m-2·s-1·Pa-1 | 参考文献 |
---|---|---|---|---|---|---|---|
Cu2(bza)4(pyz) | 2 | 尺寸差异 | 粉末MOF沉积法 | RT | 19* | 6.88×10-9 | [ |
HKUST-1 | 9 | 极化率 | 晶种法 | RT | 5.9 | 1.0×10-6 | [ |
ZIF-7 | 3 | 尺寸差异 | 晶种法 | 20~200 | 5.9 | 8.0×10-8 | [ |
ZIF-8 | 3.4 | 尺寸差异 | 晶种法 | RT | 31.5 | 2.45×10-8 | [ |
ZIF-8 | 3.4 | 尺寸差异 | 晶种法 | RT | 4.0 | 4.80×10-7 | [ |
ZIF-8 | 3.4 | 尺寸差异 | 溶剂热法 | RT | 11.2 | 6.70×10-8 | [ |
ZIF-9 | 2.4 | 尺寸差异 | 非同源金属诱导 | RT | 7.6*/6.6 | 1.80×10-7 | [ |
ZIF-22 | 3 | 尺寸差异 | 溶剂热法 | 50 | 5.2 | 1.60×10-7 | [ |
ZIF-67 | 3.4 | 尺寸差异 | 非同源金属诱导 | RT | 45.4*/41.8 | 2.30×10-7 | [ |
ZIF-67 | 3.4 | 尺寸差异 | 非同源金属诱导 | RT | 6.6* | 2.48×10-7 | [ |
ZIF-90 | 3.5 | 尺寸差异 | 晶种法 | 25~225 | 15.3 | 2.50×10-7 | [ |
UiO-66 | 6 | 尺寸差异 | 溶剂热法 | RT | 3.9* | 6.11×10-8 | [ |
分离材料 | 孔径/Å | 设计原理 | 制备方法 | 分离条件/℃ | H2/CH4选择性 | H2通量/mol·m-2·s-1·Pa-1 | 参考文献 |
---|---|---|---|---|---|---|---|
Cu2(bza)4(pyz) | 2 | 尺寸差异 | 粉末MOF沉积法 | RT | 19* | 6.88×10-9 | [ |
HKUST-1 | 9 | 极化率 | 晶种法 | RT | 5.9 | 1.0×10-6 | [ |
ZIF-7 | 3 | 尺寸差异 | 晶种法 | 20~200 | 5.9 | 8.0×10-8 | [ |
ZIF-8 | 3.4 | 尺寸差异 | 晶种法 | RT | 31.5 | 2.45×10-8 | [ |
ZIF-8 | 3.4 | 尺寸差异 | 晶种法 | RT | 4.0 | 4.80×10-7 | [ |
ZIF-8 | 3.4 | 尺寸差异 | 溶剂热法 | RT | 11.2 | 6.70×10-8 | [ |
ZIF-9 | 2.4 | 尺寸差异 | 非同源金属诱导 | RT | 7.6*/6.6 | 1.80×10-7 | [ |
ZIF-22 | 3 | 尺寸差异 | 溶剂热法 | 50 | 5.2 | 1.60×10-7 | [ |
ZIF-67 | 3.4 | 尺寸差异 | 非同源金属诱导 | RT | 45.4*/41.8 | 2.30×10-7 | [ |
ZIF-67 | 3.4 | 尺寸差异 | 非同源金属诱导 | RT | 6.6* | 2.48×10-7 | [ |
ZIF-90 | 3.5 | 尺寸差异 | 晶种法 | 25~225 | 15.3 | 2.50×10-7 | [ |
UiO-66 | 6 | 尺寸差异 | 溶剂热法 | RT | 3.9* | 6.11×10-8 | [ |
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