Chemical Industry and Engineering Progress ›› 2019, Vol. 38 ›› Issue (07): 3207-3226.DOI: 10.16085/j.issn.1000-6613.2018-1858
• Materials science and technology • Previous Articles Next Articles
Xiao ZHANG(),Yaohua XU,Hao LIU,Feng WEI,Peng YUAN
Received:
2018-09-14
Online:
2019-07-05
Published:
2019-07-05
作者简介:
张晓(1991—),女,硕士,助理工程师,研究方向为金属-有机框架材料、金属氧化物材料及其催化性能。E-mail:<email>zhangxiao@grinm.com</email>。
CLC Number:
Xiao ZHANG, Yaohua XU, Hao LIU, Feng WEI, Peng YUAN. Recent advances of ethanol detection materials based on metal oxides[J]. Chemical Industry and Engineering Progress, 2019, 38(07): 3207-3226.
张晓, 徐瑶华, 刘皓, 魏峰, 苑鹏. 基于金属氧化物的乙醇检测气敏材料的研究进展[J]. 化工进展, 2019, 38(07): 3207-3226.
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URL: https://hgjz.cip.com.cn/EN/10.16085/j.issn.1000-6613.2018-1858
材料 | 形貌 | 材料 | 温度/℃ | 检测浓度 /μg?g-1 | 响应度 | 响应/恢复(时间)/s | 选择性(响应度) | 参考文献 | |||
---|---|---|---|---|---|---|---|---|---|---|---|
甲醇 | 甲醛 | 丙酮 | 氢气 | ||||||||
零维材料 | 立方颗粒 | Co3O4 | 200 | 100 | 5.0 | 无 | 3.0 | [ | |||
团聚颗粒 | Co3O4 | 300 | 100 | 5.5 | 150/55 | 5.1 | [ | ||||
纳米颗粒 | ZnO | 350 | 400 | 20.3 | 12/14 | 无 | [ | ||||
立方颗粒 | In2O3 | 200 | 100 | 17.0 | 无 | 5.0 | [ | ||||
一维材料 | 纳米纤维 | SnO2 | 330 | 10 | 4.5 | 13/13.9 | 无 | [ | |||
纳米线 | SnO2 | 380 | 100 | 17.0 | 22/18 | 无 | [ | ||||
纳米棒 | ZnO | 400 | 100 | 149.2 | 9/15 | 无 | [ | ||||
纳米线 | Co3O4 | 350 | 300 | 5.1 | 无 | 无 | [ | ||||
纳米棒 | Co3O4 | 160 | 500 | 71.0 | 90/60 | 38.8 | 20.1 | [ | |||
纳米棒 | Co3O4 | 300 | 100 | 25.7 | 29/13 | 20.1 | [ | ||||
纳米管 | Co3O4 | 300 | 100 | 24.7 | 49/13 | 26.3 | [ | ||||
纳米纤维 | TiO2 | 300 | 100 | 14.0 | 3/5 | 3.5 | [ | ||||
二维材料 | 纳米片 | ZnO | 350 | 400 | 23.3 | 12/5 | 无 | [ | |||
纳米片 | Co3O4 | 100 | 300 | 419.0 | 44/328 | 94.0 | 36.4 | 234.0 | [ | ||
纳米片 | Co3O4 | 300 | 100 | 57.5 | 66/10 | 56.0 | [ | ||||
层状结构 | CuO | 250 | 5 | 3.1 | 11.9/8.4 | 3.0 | 1.6 | 2.5 | [ | ||
三维材料 | 分级结构 | SnO2 | 350 | 100 | 10.5 | 5 | 无 | [ | |||
介孔材料 | SnO2 | 225 | 100 | 17.3 | 8/780 | 2.5 | 2.5 | 3.0 | [ | ||
分级多孔 | SnO2 | 240 | 500 | 72.0 | 10/15 | 12.0 | 9.0 | 7.0 | [ | ||
(20μg?g-1) | |||||||||||
空心笼状 | ZnO | 300 | 1 | 8.0 | 无 | 14.8 | [ | ||||
介孔材料 | ZnO | 室温 | 300 | 1.4 | 42/40 | 无 | [ | ||||
分级多孔 | ZnO | 250 | 50 | 36.6 | 14/8 | 3.0 | [ | ||||
分级多孔 | ZnO | 220 | 100 | 8.5 | 10/80 | 5.0 | [ | ||||
分级结构 | ZnO | 370 | 100 | 340.0 | 12/约50 | 362.0 | [ | ||||
分级结构 | ZnO | 260 | 50 | 110.0 | 4/12 | 12.0 | 40.0 | 2.0 | [ | ||
纳米花 | ZnO | 350 | 400 | 30.4 | 10/4 | 无 | [ | ||||
三维微孔 | Co3O4@C | 170 | 100 | 14.7 | 无 | 11.0 | 7.8 | [ | |||
三维介孔 | Co3O4@CF | 320 | 100 | 4.2 | 44/31 | 无 | [ | ||||
介孔纳米片 | Co3O4/NCF | 100 | 100 | 10.4 | 45/140 | 1.7 | 1.6 | 1.3 | [ | ||
薄膜 | 薄膜 | SnO2 | 300 | 300 | 1.84 | 8/340 | 70.0 | [ | |||
薄膜 | ZnO | 室温 | 30 | 6.0 | 28/49 | 5.1 (10μg?g-1) | [ | ||||
薄膜 | ZnO | 400 | 50 | 55.0 | 362/147 | 无 | [ | ||||
阵列 | Co3O4 | 130 | 100 | 89.6 | 无 | 25.8 | 55.2 | [ | |||
薄膜 | CuO | 室温 | 200 | 1.24 | 15/15 | 无 | [ |
材料 | 形貌 | 材料 | 温度/℃ | 检测浓度 /μg?g-1 | 响应度 | 响应/恢复(时间)/s | 选择性(响应度) | 参考文献 | |||
---|---|---|---|---|---|---|---|---|---|---|---|
甲醇 | 甲醛 | 丙酮 | 氢气 | ||||||||
零维材料 | 立方颗粒 | Co3O4 | 200 | 100 | 5.0 | 无 | 3.0 | [ | |||
团聚颗粒 | Co3O4 | 300 | 100 | 5.5 | 150/55 | 5.1 | [ | ||||
纳米颗粒 | ZnO | 350 | 400 | 20.3 | 12/14 | 无 | [ | ||||
立方颗粒 | In2O3 | 200 | 100 | 17.0 | 无 | 5.0 | [ | ||||
一维材料 | 纳米纤维 | SnO2 | 330 | 10 | 4.5 | 13/13.9 | 无 | [ | |||
纳米线 | SnO2 | 380 | 100 | 17.0 | 22/18 | 无 | [ | ||||
纳米棒 | ZnO | 400 | 100 | 149.2 | 9/15 | 无 | [ | ||||
纳米线 | Co3O4 | 350 | 300 | 5.1 | 无 | 无 | [ | ||||
纳米棒 | Co3O4 | 160 | 500 | 71.0 | 90/60 | 38.8 | 20.1 | [ | |||
纳米棒 | Co3O4 | 300 | 100 | 25.7 | 29/13 | 20.1 | [ | ||||
纳米管 | Co3O4 | 300 | 100 | 24.7 | 49/13 | 26.3 | [ | ||||
纳米纤维 | TiO2 | 300 | 100 | 14.0 | 3/5 | 3.5 | [ | ||||
二维材料 | 纳米片 | ZnO | 350 | 400 | 23.3 | 12/5 | 无 | [ | |||
纳米片 | Co3O4 | 100 | 300 | 419.0 | 44/328 | 94.0 | 36.4 | 234.0 | [ | ||
纳米片 | Co3O4 | 300 | 100 | 57.5 | 66/10 | 56.0 | [ | ||||
层状结构 | CuO | 250 | 5 | 3.1 | 11.9/8.4 | 3.0 | 1.6 | 2.5 | [ | ||
三维材料 | 分级结构 | SnO2 | 350 | 100 | 10.5 | 5 | 无 | [ | |||
介孔材料 | SnO2 | 225 | 100 | 17.3 | 8/780 | 2.5 | 2.5 | 3.0 | [ | ||
分级多孔 | SnO2 | 240 | 500 | 72.0 | 10/15 | 12.0 | 9.0 | 7.0 | [ | ||
(20μg?g-1) | |||||||||||
空心笼状 | ZnO | 300 | 1 | 8.0 | 无 | 14.8 | [ | ||||
介孔材料 | ZnO | 室温 | 300 | 1.4 | 42/40 | 无 | [ | ||||
分级多孔 | ZnO | 250 | 50 | 36.6 | 14/8 | 3.0 | [ | ||||
分级多孔 | ZnO | 220 | 100 | 8.5 | 10/80 | 5.0 | [ | ||||
分级结构 | ZnO | 370 | 100 | 340.0 | 12/约50 | 362.0 | [ | ||||
分级结构 | ZnO | 260 | 50 | 110.0 | 4/12 | 12.0 | 40.0 | 2.0 | [ | ||
纳米花 | ZnO | 350 | 400 | 30.4 | 10/4 | 无 | [ | ||||
三维微孔 | Co3O4@C | 170 | 100 | 14.7 | 无 | 11.0 | 7.8 | [ | |||
三维介孔 | Co3O4@CF | 320 | 100 | 4.2 | 44/31 | 无 | [ | ||||
介孔纳米片 | Co3O4/NCF | 100 | 100 | 10.4 | 45/140 | 1.7 | 1.6 | 1.3 | [ | ||
薄膜 | 薄膜 | SnO2 | 300 | 300 | 1.84 | 8/340 | 70.0 | [ | |||
薄膜 | ZnO | 室温 | 30 | 6.0 | 28/49 | 5.1 (10μg?g-1) | [ | ||||
薄膜 | ZnO | 400 | 50 | 55.0 | 362/147 | 无 | [ | ||||
阵列 | Co3O4 | 130 | 100 | 89.6 | 无 | 25.8 | 55.2 | [ | |||
薄膜 | CuO | 室温 | 200 | 1.24 | 15/15 | 无 | [ |
掺杂物 | 形貌 | 材料 | 温度 /℃ | 检测浓度 /μg?g-1 | 响应度 | 响应/恢复(时间)/s | 选择性(响应度) | 参考 文献 | |||
---|---|---|---|---|---|---|---|---|---|---|---|
甲醇 | 甲醛 | 丙酮 | 氨气 | ||||||||
贵金属 | 中空纳米球 | Pt-SnO2 | 325 | 5 | 1399.9 | 1/525 | 600.0 | 700.0 | 200 | [ | |
纳米棒 | Pt-SnO2 | 320 | 200 | 8.3 | 3~5/5~15 | 无 | [ | ||||
纳米颗粒 | Pt-SnO2 | 275 | 100 | 1.9 | 1/5 | 无 | [ | ||||
空心材料 | Pd-SnO2 | 300 | 50 | 2.0 | 1.5/18 | 0.9 | 0.9 | 1.0 | [ | ||
纳米花 | Au-SnO2 | 340 | 150 | 29.3 | 5/10 | 13.3 | 20.3 | [ | |||
(100μg·g-1) | |||||||||||
薄膜 | Pt-In2O3 | 室温 | 0.095 | 12.2 | 1/2 | 无 | [ | ||||
纳米颗粒 | Pt-In2O3 | 250 | 100 | 32.6 | 2.2/0.7 | 4.0 | [ | ||||
纳米片 | Au-WO3 | 320 | 100 | 97.2 | 无 | 8.0 | 3.0 | 11.0 | [ | ||
非贵金属 | 纳米颗粒 | CuZn-SnO2 | 110 | 50 | 210.0 | 无 | 10.0 | [ | |||
纳米棒 | Ni-SnO2 | 450 | 50 | 2000.0 | 30/600 | 无 | [ | ||||
纳米微球 | Ni-SnO2 | 260 | 100 | 28.9 | 11/54 | 6.0 | 4.0 | [ | |||
纳米颗粒 | Ce-SnO2 | 室温 | 400 | 4.8 | 2~25/30~60 | 无 | [ | ||||
立方中空 | ZnSnO3 | 260 | 100 | 34.1 | 2/276 | 11.0 | 3 | [ | |||
纳米棒 | Cr-ZnO | 300 | 400 | 45.0 | 无 | 无 | [ | ||||
海绵状 | Co-ZnO | 220 | 100 | 120.0 | 10/5 | 18.0 | 24.0 | [ | |||
六边形 | Cr-Co3O4 | 300 | 100 | 28.9 | 1/7 | 4.0 | 3.0 | [ | |||
纳米球 | Co3O4/pCNH | 210 | 500 | 30.2 | 无 | 2.0 | 7.0 | [ |
掺杂物 | 形貌 | 材料 | 温度 /℃ | 检测浓度 /μg?g-1 | 响应度 | 响应/恢复(时间)/s | 选择性(响应度) | 参考 文献 | |||
---|---|---|---|---|---|---|---|---|---|---|---|
甲醇 | 甲醛 | 丙酮 | 氨气 | ||||||||
贵金属 | 中空纳米球 | Pt-SnO2 | 325 | 5 | 1399.9 | 1/525 | 600.0 | 700.0 | 200 | [ | |
纳米棒 | Pt-SnO2 | 320 | 200 | 8.3 | 3~5/5~15 | 无 | [ | ||||
纳米颗粒 | Pt-SnO2 | 275 | 100 | 1.9 | 1/5 | 无 | [ | ||||
空心材料 | Pd-SnO2 | 300 | 50 | 2.0 | 1.5/18 | 0.9 | 0.9 | 1.0 | [ | ||
纳米花 | Au-SnO2 | 340 | 150 | 29.3 | 5/10 | 13.3 | 20.3 | [ | |||
(100μg·g-1) | |||||||||||
薄膜 | Pt-In2O3 | 室温 | 0.095 | 12.2 | 1/2 | 无 | [ | ||||
纳米颗粒 | Pt-In2O3 | 250 | 100 | 32.6 | 2.2/0.7 | 4.0 | [ | ||||
纳米片 | Au-WO3 | 320 | 100 | 97.2 | 无 | 8.0 | 3.0 | 11.0 | [ | ||
非贵金属 | 纳米颗粒 | CuZn-SnO2 | 110 | 50 | 210.0 | 无 | 10.0 | [ | |||
纳米棒 | Ni-SnO2 | 450 | 50 | 2000.0 | 30/600 | 无 | [ | ||||
纳米微球 | Ni-SnO2 | 260 | 100 | 28.9 | 11/54 | 6.0 | 4.0 | [ | |||
纳米颗粒 | Ce-SnO2 | 室温 | 400 | 4.8 | 2~25/30~60 | 无 | [ | ||||
立方中空 | ZnSnO3 | 260 | 100 | 34.1 | 2/276 | 11.0 | 3 | [ | |||
纳米棒 | Cr-ZnO | 300 | 400 | 45.0 | 无 | 无 | [ | ||||
海绵状 | Co-ZnO | 220 | 100 | 120.0 | 10/5 | 18.0 | 24.0 | [ | |||
六边形 | Cr-Co3O4 | 300 | 100 | 28.9 | 1/7 | 4.0 | 3.0 | [ | |||
纳米球 | Co3O4/pCNH | 210 | 500 | 30.2 | 无 | 2.0 | 7.0 | [ |
异质结 | 材料 | 温度/℃ | 检测浓度/μg?g-1 | 响应度 | 响应/恢复时间/s | 选择性(响应度) | 参考 文献 | |||
---|---|---|---|---|---|---|---|---|---|---|
甲醇 | 甲醛 | 丙酮 | 氨气 | |||||||
MO x -MO x | ZnO/SnO2 | 225 | 30 | 34.8 | 1/120 | 53.7 | 8.9 | 52.1 | [ | |
(100μg?g-1, 此时乙醇响应度为78.2) | ||||||||||
NiO/SnO2 | 250 | 100 | 7.9 | 15/100 | 无 | [ | ||||
Fe2O3/SnO2 | 300 | 200 | 57.6 | 无 | 20.0 | 15.0 | 35.0 | [ | ||
CoO/SnO2 | 250 | 100 | 145.0 | 无 | 56.0 | 15.0 | 54.0 | [ | ||
SnO2/ZnO | 350 | 100 | 13.3 | 无 | 4.0 | 4.0 | 1.4 | [ | ||
SnO2/Fe2O3 | 260 | 100 | 41.7 | 3/4 | 9.0 | 5.0 | [ | |||
SnO2/Fe2O3 | 240 | 100 | 5.9 | 1/5 | 1.0 | 2.5 | 1.5 | [ | ||
ZnO/CuO | 300 | 10 | 2.2 | 22/26 | 1.2 | 0.7 | [ | |||
ZnO/Co3O4 | 200 | 1000 | 106.0 | 7/236 | 无 | [ | ||||
LaMnO3/ZnO | 300 | 50 | 6.0 | 8/17 | 无 | [ | ||||
CuO/ZnO | 320 | 200 | 97.0 | 5/25 | 57.0 | 20.0 | [ | |||
CdO/ZnO | 250 | 100 | 65.5 | 2/136 | 10.0 | 9.0 | 15.0 | [ | ||
CdO/Mn-ZnO | 340 | 20 | 11.4 | 11.4/12.4 | 2.0 | 1.2 | [ | |||
α-Fe2O3/ZnO/Au | 280 | 100 | 170.0 | 4/5 | 无 | [ | ||||
MoO3/WO3 | 320 | 100 | 28.5 | 13/10 | 18.2 | [ | ||||
Cr2O3/WO3 | 300 | 200 | 5.6 | 约46/57 | 4.1 | [ | ||||
MoO3/In2O3 | 185 | 100 | 7.0 | 11/94 | 2.5 | [ | ||||
有机材料&石墨烯/MO x | PANI/TiO2 | 室温 | 200 | 约47.0 | 115/340 | 无 | [ | |||
Zn2SnO4/rGO | 275 | 100 | 38.0 | 11/18 | 15.0 | 3.5 | 16 | [ | ||
rGO-SnO2 | 300 | 100 | 70.4 | 11/ | 42.0 | 13 | [ | |||
Fe3O4/rGO | 400 | 100 | 9.0 | 3/138 | 1.100 | [ | ||||
TiO2[/多孔硅 | 150 | 100 | 1.4 | 无 | 1.03 | [ |
异质结 | 材料 | 温度/℃ | 检测浓度/μg?g-1 | 响应度 | 响应/恢复时间/s | 选择性(响应度) | 参考 文献 | |||
---|---|---|---|---|---|---|---|---|---|---|
甲醇 | 甲醛 | 丙酮 | 氨气 | |||||||
MO x -MO x | ZnO/SnO2 | 225 | 30 | 34.8 | 1/120 | 53.7 | 8.9 | 52.1 | [ | |
(100μg?g-1, 此时乙醇响应度为78.2) | ||||||||||
NiO/SnO2 | 250 | 100 | 7.9 | 15/100 | 无 | [ | ||||
Fe2O3/SnO2 | 300 | 200 | 57.6 | 无 | 20.0 | 15.0 | 35.0 | [ | ||
CoO/SnO2 | 250 | 100 | 145.0 | 无 | 56.0 | 15.0 | 54.0 | [ | ||
SnO2/ZnO | 350 | 100 | 13.3 | 无 | 4.0 | 4.0 | 1.4 | [ | ||
SnO2/Fe2O3 | 260 | 100 | 41.7 | 3/4 | 9.0 | 5.0 | [ | |||
SnO2/Fe2O3 | 240 | 100 | 5.9 | 1/5 | 1.0 | 2.5 | 1.5 | [ | ||
ZnO/CuO | 300 | 10 | 2.2 | 22/26 | 1.2 | 0.7 | [ | |||
ZnO/Co3O4 | 200 | 1000 | 106.0 | 7/236 | 无 | [ | ||||
LaMnO3/ZnO | 300 | 50 | 6.0 | 8/17 | 无 | [ | ||||
CuO/ZnO | 320 | 200 | 97.0 | 5/25 | 57.0 | 20.0 | [ | |||
CdO/ZnO | 250 | 100 | 65.5 | 2/136 | 10.0 | 9.0 | 15.0 | [ | ||
CdO/Mn-ZnO | 340 | 20 | 11.4 | 11.4/12.4 | 2.0 | 1.2 | [ | |||
α-Fe2O3/ZnO/Au | 280 | 100 | 170.0 | 4/5 | 无 | [ | ||||
MoO3/WO3 | 320 | 100 | 28.5 | 13/10 | 18.2 | [ | ||||
Cr2O3/WO3 | 300 | 200 | 5.6 | 约46/57 | 4.1 | [ | ||||
MoO3/In2O3 | 185 | 100 | 7.0 | 11/94 | 2.5 | [ | ||||
有机材料&石墨烯/MO x | PANI/TiO2 | 室温 | 200 | 约47.0 | 115/340 | 无 | [ | |||
Zn2SnO4/rGO | 275 | 100 | 38.0 | 11/18 | 15.0 | 3.5 | 16 | [ | ||
rGO-SnO2 | 300 | 100 | 70.4 | 11/ | 42.0 | 13 | [ | |||
Fe3O4/rGO | 400 | 100 | 9.0 | 3/138 | 1.100 | [ | ||||
TiO2[/多孔硅 | 150 | 100 | 1.4 | 无 | 1.03 | [ |
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