Chemical Industry and Engineering Progress ›› 2022, Vol. 41 ›› Issue (6): 3235-3248.DOI: 10.16085/j.issn.1000-6613.2021-1365
• Resources and environmental engineering • Previous Articles Next Articles
LIAO Bing1,2,3(), XU Wen1,2,3, YE Qiuyue1,2,3
Received:
2021-06-29
Revised:
2021-08-08
Online:
2022-06-21
Published:
2022-06-10
Contact:
LIAO Bing
通讯作者:
廖兵
作者简介:
廖兵(1989—),男,副教授,硕士生导师,研究方向为水土污染控制与修复。E-mail:基金资助:
CLC Number:
LIAO Bing, XU Wen, YE Qiuyue. A review of activated percarbonate and peroxymonocarbonate in the field of water treatment[J]. Chemical Industry and Engineering Progress, 2022, 41(6): 3235-3248.
廖兵, 胥雯, 叶秋月. 活化过碳酸盐及过氧碳酸氢盐在水处理领域中的研究进展[J]. 化工进展, 2022, 41(6): 3235-3248.
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活化类型 | 活化剂 | 活化剂浓度 | 目标污染物 | 污染物浓度 | 反应时间 /min | 降解率 /% | 参考 文献 |
---|---|---|---|---|---|---|---|
铁基材料 | Fe(Ⅱ) | 1.0mmol/L | PCE | 0.12mmol/L | 1 | 90 | [ |
Fe(Ⅱ) | 0.3mmol/L | SMT | 0.02mmol/L | 1 | 84 | [ | |
Fe(Ⅲ) | 1.0mmol/L | PCE | 0.12mmol/L | 60 | 28 | [ | |
Fe2+ | 3.0mmol/L | 苯 | 1.0mmol/L | 20 | 100 | [ | |
CIT-Fe2+ | 1mmol/L、5mmol/L | PCE | 0.12mmol/L | 20 | 99.99 | [ | |
OA-Fe2+ | 5mmol/L、5mmol/L | PCE | 0.12mmol/L | 20 | >90 | [ | |
CA-Fe2+ | 1.0mmol/L、0.45mmol/L | TCE | 0.15mmol/L | 90 | 98 | [ | |
CIA-Fe2+ | 1mmol/L、2mmol/L | 苯 | 1mmol/L | 30 | 96.3 | [ | |
Z-nZVI-Ni | 250mg/L | TCE | 0.15mmol/L | 180 | 99.8 | [ | |
Z-nZVI-Cu | 200mg/L | TCE | 0.15mmol/L | 180 | >95 | [ | |
G-nZVI | 0.8g/L | 1,1,1-三氯乙烷(TCA) | 0.15mmol/L | 120 | 90 | [ | |
NZ-nZVI | — | 酸橙52(AO52) | 25mg/L | 18 | 100 | [ | |
生物炭 | 红藻生物炭 | 3.0g/L | 邻苯二甲酸二(2-乙基己基)酯(DEHP) | 0.02mmol/L | 12 | 63 | [ |
富含铁锰的生物炭 | 1.67g/L | 多环芳烃(PAHs) | 1.67g/L | 6 | >80 | [ | |
光活化 | UV | — | 2-羟基-4-甲氧基二苯甲酮(BP-3) | 0.02mmol/L | 180 | >78 | [ |
UV | 0.1mW·cm-2 | 双酚A(BPA) | 0.002mmol/L | — | 87.8 | [ | |
其他 | Fe3O4@ZIF-8 | 1g/L | 亚甲蓝(MB) | 20mg/L | 120 | 98.5 | [ |
FeOCl/vis | 0.5g/L | 罗丹明B(RhB) | 20mg/L | 60 | 95.8 | [ | |
V(Ⅳ) | 1.0mmol/L | 苯胺 | 1.0mmol/L | 15 | 55.62 | [ | |
VOSO4 | 1.0mmol/L | 苯胺 | 1.0mmol/L | 15 | 41.29 | [ |
活化类型 | 活化剂 | 活化剂浓度 | 目标污染物 | 污染物浓度 | 反应时间 /min | 降解率 /% | 参考 文献 |
---|---|---|---|---|---|---|---|
铁基材料 | Fe(Ⅱ) | 1.0mmol/L | PCE | 0.12mmol/L | 1 | 90 | [ |
Fe(Ⅱ) | 0.3mmol/L | SMT | 0.02mmol/L | 1 | 84 | [ | |
Fe(Ⅲ) | 1.0mmol/L | PCE | 0.12mmol/L | 60 | 28 | [ | |
Fe2+ | 3.0mmol/L | 苯 | 1.0mmol/L | 20 | 100 | [ | |
CIT-Fe2+ | 1mmol/L、5mmol/L | PCE | 0.12mmol/L | 20 | 99.99 | [ | |
OA-Fe2+ | 5mmol/L、5mmol/L | PCE | 0.12mmol/L | 20 | >90 | [ | |
CA-Fe2+ | 1.0mmol/L、0.45mmol/L | TCE | 0.15mmol/L | 90 | 98 | [ | |
CIA-Fe2+ | 1mmol/L、2mmol/L | 苯 | 1mmol/L | 30 | 96.3 | [ | |
Z-nZVI-Ni | 250mg/L | TCE | 0.15mmol/L | 180 | 99.8 | [ | |
Z-nZVI-Cu | 200mg/L | TCE | 0.15mmol/L | 180 | >95 | [ | |
G-nZVI | 0.8g/L | 1,1,1-三氯乙烷(TCA) | 0.15mmol/L | 120 | 90 | [ | |
NZ-nZVI | — | 酸橙52(AO52) | 25mg/L | 18 | 100 | [ | |
生物炭 | 红藻生物炭 | 3.0g/L | 邻苯二甲酸二(2-乙基己基)酯(DEHP) | 0.02mmol/L | 12 | 63 | [ |
富含铁锰的生物炭 | 1.67g/L | 多环芳烃(PAHs) | 1.67g/L | 6 | >80 | [ | |
光活化 | UV | — | 2-羟基-4-甲氧基二苯甲酮(BP-3) | 0.02mmol/L | 180 | >78 | [ |
UV | 0.1mW·cm-2 | 双酚A(BPA) | 0.002mmol/L | — | 87.8 | [ | |
其他 | Fe3O4@ZIF-8 | 1g/L | 亚甲蓝(MB) | 20mg/L | 120 | 98.5 | [ |
FeOCl/vis | 0.5g/L | 罗丹明B(RhB) | 20mg/L | 60 | 95.8 | [ | |
V(Ⅳ) | 1.0mmol/L | 苯胺 | 1.0mmol/L | 15 | 55.62 | [ | |
VOSO4 | 1.0mmol/L | 苯胺 | 1.0mmol/L | 15 | 41.29 | [ |
活化类型 | 活化剂 | 活化剂浓度/投加量 | 目标污染物 | 污染物浓度 | 反应时间/min | 降解率/% | 参考文献 |
---|---|---|---|---|---|---|---|
过渡金属离子 | Co2+ | 0.02mmol/L | MB | 0.134mmol/L | 50 | 100 | [ |
Co2+ | 0.005mmol/L | 酸性橙Ⅱ(AOII) | 0.05mmol/L | 10 | >90 | [ | |
Co2+ | 0.005mmol/L | AOII | 0.25mmol/L | 180 | >90 | [ | |
Cu(Ⅱ) | 0.03mmol/L | AOII | 0.05mmol/L | 10 | >90 | [ | |
Cu(Ⅱ) | 0.01mmol/L | 三氯生(TCS) | 0.01mmol/L | 40 | >65 | [ | |
复合材料 | S-CoFe2O4 | 0.1g/L | AOII | 50mg/L | 60 | 98 | [ |
CoMgAl | 0.03g | 亚甲基橙(MO) | 49.8mg/L | 60 | >95 | [ | |
CuFeS2 | 200mg/L | 2,4-DCP | 10mg/L | 120 | >80 | [ | |
Co x Mn3-x O4 | 0.1g/L | 2,4-DCP | 10mg/L | 120 | >85 | [ |
活化类型 | 活化剂 | 活化剂浓度/投加量 | 目标污染物 | 污染物浓度 | 反应时间/min | 降解率/% | 参考文献 |
---|---|---|---|---|---|---|---|
过渡金属离子 | Co2+ | 0.02mmol/L | MB | 0.134mmol/L | 50 | 100 | [ |
Co2+ | 0.005mmol/L | 酸性橙Ⅱ(AOII) | 0.05mmol/L | 10 | >90 | [ | |
Co2+ | 0.005mmol/L | AOII | 0.25mmol/L | 180 | >90 | [ | |
Cu(Ⅱ) | 0.03mmol/L | AOII | 0.05mmol/L | 10 | >90 | [ | |
Cu(Ⅱ) | 0.01mmol/L | 三氯生(TCS) | 0.01mmol/L | 40 | >65 | [ | |
复合材料 | S-CoFe2O4 | 0.1g/L | AOII | 50mg/L | 60 | 98 | [ |
CoMgAl | 0.03g | 亚甲基橙(MO) | 49.8mg/L | 60 | >95 | [ | |
CuFeS2 | 200mg/L | 2,4-DCP | 10mg/L | 120 | >80 | [ | |
Co x Mn3-x O4 | 0.1g/L | 2,4-DCP | 10mg/L | 120 | >85 | [ |
活化剂 | 污染物 | 初始pH | 反应后pH | 降解率/% | 参考文献 |
---|---|---|---|---|---|
Fe(Ⅱ) | SMT | 4.0 | 3.05 | 88 | [ |
CA-Fe2+ | TCE | 3.01 | 2.85 | 93 | [ |
Fe3O4@ZIF-8 | MB | 3 | — | 98.5 | [ |
CA-Fe(Ⅱ) | TCE | 3.0 | 2.9 | 93.1 | [ |
HAH/CA-Fe(Ⅱ) | TCE | 3 | 2.5 | >99 | [ |
CIT/Fe(Ⅱ) | PCE | <4 | 3.35 | 92.6 | [ |
nZVI | BPA | 3 | — | 100 | [ |
Fe2+ | PCE | 6.5 | 3.44 | 98 | [ |
g-C3N4/Vis | MB | 7 | — | 90 | [ |
富含铁锰的生物炭 | PAHs | 11.0 | — | 85 | [ |
O3 | SMX | 10.3 | 8.0 | >70 | [ |
活化剂 | 污染物 | 初始pH | 反应后pH | 降解率/% | 参考文献 |
---|---|---|---|---|---|
Fe(Ⅱ) | SMT | 4.0 | 3.05 | 88 | [ |
CA-Fe2+ | TCE | 3.01 | 2.85 | 93 | [ |
Fe3O4@ZIF-8 | MB | 3 | — | 98.5 | [ |
CA-Fe(Ⅱ) | TCE | 3.0 | 2.9 | 93.1 | [ |
HAH/CA-Fe(Ⅱ) | TCE | 3 | 2.5 | >99 | [ |
CIT/Fe(Ⅱ) | PCE | <4 | 3.35 | 92.6 | [ |
nZVI | BPA | 3 | — | 100 | [ |
Fe2+ | PCE | 6.5 | 3.44 | 98 | [ |
g-C3N4/Vis | MB | 7 | — | 90 | [ |
富含铁锰的生物炭 | PAHs | 11.0 | — | 85 | [ |
O3 | SMX | 10.3 | 8.0 | >70 | [ |
活化类型 | 反应式 | 编号 | 参考文献 |
---|---|---|---|
铁基材料 | H2O2 + Fe(Ⅱ) | (8) | [ |
HO·+ H2O2 | (9) | ||
HO·+ Fe(Ⅱ) | (10) | ||
COOH- + HO· | (11) | [ | |
COOH- + H· | (12) | ||
HO· + HO· | (13) | [ | |
HO·+ Fe(Ⅱ) | (10) | ||
H2O2 + HO· | (14) | ||
HO· + CO | (7) | [ | |
HO· + HCO | (15) | ||
Fe0 + O2 + 2H+ | (16) | ||
Fe0 + H2O2 + 2H+ | (17) | ||
Fe2+ + H2O2 | (18) | ||
2Fe3+ + Fe0 | (19) | ||
Ni+ + H2O2 | (20) | [ | |
Ni2+ + H2O2 | (21) | ||
Fe3+ + Ni+ | (22) | ||
生物炭材料 | RSB-π+ +H2O2 | (23) | [ |
Fe3+ + H2O2 | (24) | [ | |
Fe3+ + O | (25) | ||
Fe3+ + HO2· | (26) | ||
Mn2+ + H2O2 | (27) | ||
Mn3+ + H2O2 | (28) | ||
Mn3+ + H2O2 | (29) | ||
Mn3+ + O | (30) | ||
Mn3+ + HO2· | (31) | ||
Fe2+ + Mn3+ | (32) | ||
PAHs + HO· + O | (33) | ||
光活化 | H2O2 + hv | (34) | [ |
HO· + HCO3- | (15) | [ | |
HO· + CO32- | (7) | ||
其他 | VO2+ + H2O | (35) | [ |
[VOOH]+ + H2O + H2O2 | (36) | ||
HVO42- + H2O2 + 3H+ | (37) | ||
HO· + CO | (7) | ||
H2O2 + CO | (38) | ||
HO2· | (39) |
活化类型 | 反应式 | 编号 | 参考文献 |
---|---|---|---|
铁基材料 | H2O2 + Fe(Ⅱ) | (8) | [ |
HO·+ H2O2 | (9) | ||
HO·+ Fe(Ⅱ) | (10) | ||
COOH- + HO· | (11) | [ | |
COOH- + H· | (12) | ||
HO· + HO· | (13) | [ | |
HO·+ Fe(Ⅱ) | (10) | ||
H2O2 + HO· | (14) | ||
HO· + CO | (7) | [ | |
HO· + HCO | (15) | ||
Fe0 + O2 + 2H+ | (16) | ||
Fe0 + H2O2 + 2H+ | (17) | ||
Fe2+ + H2O2 | (18) | ||
2Fe3+ + Fe0 | (19) | ||
Ni+ + H2O2 | (20) | [ | |
Ni2+ + H2O2 | (21) | ||
Fe3+ + Ni+ | (22) | ||
生物炭材料 | RSB-π+ +H2O2 | (23) | [ |
Fe3+ + H2O2 | (24) | [ | |
Fe3+ + O | (25) | ||
Fe3+ + HO2· | (26) | ||
Mn2+ + H2O2 | (27) | ||
Mn3+ + H2O2 | (28) | ||
Mn3+ + H2O2 | (29) | ||
Mn3+ + O | (30) | ||
Mn3+ + HO2· | (31) | ||
Fe2+ + Mn3+ | (32) | ||
PAHs + HO· + O | (33) | ||
光活化 | H2O2 + hv | (34) | [ |
HO· + HCO3- | (15) | [ | |
HO· + CO32- | (7) | ||
其他 | VO2+ + H2O | (35) | [ |
[VOOH]+ + H2O + H2O2 | (36) | ||
HVO42- + H2O2 + 3H+ | (37) | ||
HO· + CO | (7) | ||
H2O2 + CO | (38) | ||
HO2· | (39) |
体系 | 反应式 | 编号 | 参考文献 |
---|---|---|---|
PMC | HCO | (3) | [ |
HCO | (40) | ||
HCO | (41) | ||
H2O2 + CO | (38) | ||
HO· + HO2· | (42) | ||
HO2· | (39) | ||
H2O2 | (43) | ||
O | (44) | ||
HO2· + HO2· | (45) | ||
活化PMC | HCO | (3) | [ |
≡≡ Fe(Ⅱ) + 2HCO | (52) | ||
≡≡ Fe(Ⅲ) + H2O2 | (53) | ||
CO | (54) | ||
O | (44) | ||
Co2+ + HCO | (46) | [ | |
[CoⅡ(HCO | (47) | ||
[CoⅡ(HCO | (48) | ||
[CoⅡ(HCO | (49) | ||
[CoⅢ(HCO | (50) | ||
[CoⅢ(HCO | (51) |
体系 | 反应式 | 编号 | 参考文献 |
---|---|---|---|
PMC | HCO | (3) | [ |
HCO | (40) | ||
HCO | (41) | ||
H2O2 + CO | (38) | ||
HO· + HO2· | (42) | ||
HO2· | (39) | ||
H2O2 | (43) | ||
O | (44) | ||
HO2· + HO2· | (45) | ||
活化PMC | HCO | (3) | [ |
≡≡ Fe(Ⅱ) + 2HCO | (52) | ||
≡≡ Fe(Ⅲ) + H2O2 | (53) | ||
CO | (54) | ||
O | (44) | ||
Co2+ + HCO | (46) | [ | |
[CoⅡ(HCO | (47) | ||
[CoⅡ(HCO | (48) | ||
[CoⅡ(HCO | (49) | ||
[CoⅢ(HCO | (50) | ||
[CoⅢ(HCO | (51) |
体系 | 活化类型 | 活化剂 | 污染物 | 体系中自由基种类 | 起主要作用的物质 | 参考文献 |
---|---|---|---|---|---|---|
SPC | 铁基材料 | Fe(Ⅱ) | SMX | HO·、O | HO· | [ |
Fe(Ⅱ) | PCE | [ | ||||
Fe(Ⅱ) | 苯 | [ | ||||
Fe(Ⅱ) | 四环素 | [ | ||||
Fe(Ⅲ) | 苯 | [ | ||||
螯合剂-Fe2+ | TCE | [ | ||||
Fe(Ⅱ)-CA | TCE | [ | ||||
Fe(Ⅱ)-OA | PCE | [ | ||||
FA/Fe(Ⅱ) | CT | HO·、CO | CO | [ | ||
生物炭材料 | 富含Fe、Mn的生物炭 | PAHs | O | HO· | [ | |
光活化 | UV | BP-3 | HO· | [ | ||
UV | BPA | HO·、CO | [ | |||
其他 | V(Ⅳ) | 苯胺 | HO·、O | O | [ | |
VOSO4 | 苯胺 | [ | ||||
PMC | 过渡金属 | Co2+ | MB | HO· | HO· | [ |
Co2+ | AOⅡ | 加密HO· | 加密HO· | [ | ||
Co2+ | AOⅡ | HO·、O | HO· | [ | ||
Cu(Ⅱ) | AOⅡ | HO·、O | Cu(Ⅲ) | [ | ||
Cu(Ⅱ) | TCS | O | O | [ | ||
金属复合材料 | S-CoFe2O4 | AOⅡ | 加密HO· | 加密HO· | [ | |
CoMgAl | MO | HO·、O | HO·、O | [ | ||
CuFeS2 | 2,4-DCP | HO·、1O2、O | HO·、1O2、O | [ | ||
Co x Mn3-x O4 | 2,4-DCP | HO·、O | HO·、O | [ |
体系 | 活化类型 | 活化剂 | 污染物 | 体系中自由基种类 | 起主要作用的物质 | 参考文献 |
---|---|---|---|---|---|---|
SPC | 铁基材料 | Fe(Ⅱ) | SMX | HO·、O | HO· | [ |
Fe(Ⅱ) | PCE | [ | ||||
Fe(Ⅱ) | 苯 | [ | ||||
Fe(Ⅱ) | 四环素 | [ | ||||
Fe(Ⅲ) | 苯 | [ | ||||
螯合剂-Fe2+ | TCE | [ | ||||
Fe(Ⅱ)-CA | TCE | [ | ||||
Fe(Ⅱ)-OA | PCE | [ | ||||
FA/Fe(Ⅱ) | CT | HO·、CO | CO | [ | ||
生物炭材料 | 富含Fe、Mn的生物炭 | PAHs | O | HO· | [ | |
光活化 | UV | BP-3 | HO· | [ | ||
UV | BPA | HO·、CO | [ | |||
其他 | V(Ⅳ) | 苯胺 | HO·、O | O | [ | |
VOSO4 | 苯胺 | [ | ||||
PMC | 过渡金属 | Co2+ | MB | HO· | HO· | [ |
Co2+ | AOⅡ | 加密HO· | 加密HO· | [ | ||
Co2+ | AOⅡ | HO·、O | HO· | [ | ||
Cu(Ⅱ) | AOⅡ | HO·、O | Cu(Ⅲ) | [ | ||
Cu(Ⅱ) | TCS | O | O | [ | ||
金属复合材料 | S-CoFe2O4 | AOⅡ | 加密HO· | 加密HO· | [ | |
CoMgAl | MO | HO·、O | HO·、O | [ | ||
CuFeS2 | 2,4-DCP | HO·、1O2、O | HO·、1O2、O | [ | ||
Co x Mn3-x O4 | 2,4-DCP | HO·、O | HO·、O | [ |
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