Chemical Industry and Engineering Progress ›› 2021, Vol. 40 ›› Issue (8): 4551-4561.DOI: 10.16085/j.issn.1000-6613.2020-1993
• Resources and environmental engineering • Previous Articles Next Articles
WU Wentong(), ZHANG Lingling(), LI Zifu, WANG Chenxi, YU Chunsong, WANG Qingguo
Received:
2020-09-30
Online:
2021-08-12
Published:
2021-08-05
Contact:
ZHANG Lingling
吴文瞳(), 张玲玲(), 李子富, 王晨希, 余春松, 王庆国
通讯作者:
张玲玲
作者简介:
吴文瞳(1996—),女,硕士研究生,研究方向为过硫酸盐高级氧化处理抗生素废水。E-mail:基金资助:
CLC Number:
WU Wentong, ZHANG Lingling, LI Zifu, WANG Chenxi, YU Chunsong, WANG Qingguo. Research progress of advanced oxidation technology in degradation of antibiotics and removal of antibiotic resistance[J]. Chemical Industry and Engineering Progress, 2021, 40(8): 4551-4561.
吴文瞳, 张玲玲, 李子富, 王晨希, 余春松, 王庆国. 高级氧化技术降解抗生素及去除耐药性的研究进展[J]. 化工进展, 2021, 40(8): 4551-4561.
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URL: https://hgjz.cip.com.cn/EN/10.16085/j.issn.1000-6613.2020-1993
国家 | 水生系统 | 抗生素 | ARB | ARGs | 文献 |
---|---|---|---|---|---|
中国 | 太湖流域地表水 | 四环素、土霉素等9种 | 耐药大肠杆菌 | blaCTX,sulⅠ,tet A,qnr S,aac-1b等39种 | [ |
中国 | 北京市区7条河流 | 磺胺类和四环素 | 河流细菌(耐药率0.512~0.971) | sul1,sul2,tetA,tetB,tetE,tetW,tetM,tetZ | [ |
西班牙 | 河流,污水处理厂 | 甲氧苄啶、氧氟沙星等11种 | — | qnrS,ermB,tetW,blaTEM,blaNDM,blaKPC,vanA | [ |
荷兰 | 62家污水处理厂 | — | 耐药革兰阳性细菌、大肠杆菌等 | ermB,sul1,sul2,tetM,tetM,qnrS,blaCTXM | [ |
日本 | 宫崎市城市河流 | 万古霉素 | 耐药肠球菌 | vanA,vanB,vanC1,vanC2/C3 | [ |
印度 | 医院废水, 河流 | — | 耐药大肠杆菌、肠球菌属、假单胞菌 | blaTEM,blaCTX-M,blaSHV,blaNDM,aadA | [ |
德国,澳大利亚 | 河流 | 四环素、氯霉素、磺酰胺等8种 | — | Ampc,vanA,tetA,aac(3)-IIa,dfrA1,ermA 等24种 | [ |
美国 | 河流 | β-内酰胺类抗生素 | 耐药革兰阴性菌 | — | [ |
法国 | 河流 | 四环素、阿莫西林等16种 | 耐药大肠杆菌 | — | [ |
国家 | 水生系统 | 抗生素 | ARB | ARGs | 文献 |
---|---|---|---|---|---|
中国 | 太湖流域地表水 | 四环素、土霉素等9种 | 耐药大肠杆菌 | blaCTX,sulⅠ,tet A,qnr S,aac-1b等39种 | [ |
中国 | 北京市区7条河流 | 磺胺类和四环素 | 河流细菌(耐药率0.512~0.971) | sul1,sul2,tetA,tetB,tetE,tetW,tetM,tetZ | [ |
西班牙 | 河流,污水处理厂 | 甲氧苄啶、氧氟沙星等11种 | — | qnrS,ermB,tetW,blaTEM,blaNDM,blaKPC,vanA | [ |
荷兰 | 62家污水处理厂 | — | 耐药革兰阳性细菌、大肠杆菌等 | ermB,sul1,sul2,tetM,tetM,qnrS,blaCTXM | [ |
日本 | 宫崎市城市河流 | 万古霉素 | 耐药肠球菌 | vanA,vanB,vanC1,vanC2/C3 | [ |
印度 | 医院废水, 河流 | — | 耐药大肠杆菌、肠球菌属、假单胞菌 | blaTEM,blaCTX-M,blaSHV,blaNDM,aadA | [ |
德国,澳大利亚 | 河流 | 四环素、氯霉素、磺酰胺等8种 | — | Ampc,vanA,tetA,aac(3)-IIa,dfrA1,ermA 等24种 | [ |
美国 | 河流 | β-内酰胺类抗生素 | 耐药革兰阴性菌 | — | [ |
法国 | 河流 | 四环素、阿莫西林等16种 | 耐药大肠杆菌 | — | [ |
自由基 | 半衰期/μs | 氧化电位/V | pH适用范围 |
---|---|---|---|
SO | 30~40 | 2.50~3.10 | 2~10 |
·OH | 10-3 | 2.80 | 2~9 |
自由基 | 半衰期/μs | 氧化电位/V | pH适用范围 |
---|---|---|---|
SO | 30~40 | 2.50~3.10 | 2~10 |
·OH | 10-3 | 2.80 | 2~9 |
改性方式 | 改性材料 | 抗生素 | 降解率 | 主要自由基 | 文献 |
---|---|---|---|---|---|
纳米改性 | 纳米Fe0 | 磺胺甲唑 | 87.6% | ·OH(pH>8.5) | [ |
纳米Fe0 | 磺胺嘧啶 | 93% | — | [ | |
双金属体系 | Fe0/Ag | 左氧氟沙星 氯霉素 | 60% 91% | SO | [ |
纳米Fe0/Cu | 盐酸四环素 | 89% | SO | [ | |
预处理 | 超声 | 磺胺嘧啶 | 95.7% | SO | [ |
预磁化 | 磺胺嘧啶 | 49.3% | SO | [ | |
水热 | 氯霉素 | 70.89% | — | [ | |
材料负载 | 介孔炭负载纳米Fe0 | 四环素 | 92.1% | SO | [ |
生物炭负载Fe0/Ni | 诺氟沙星 | 90%以上 | SO | [ | |
硫化改性 | 硫化纳米Fe0 | 磺胺嘧啶 | 100% | — | [ |
硫化纳米Fe0/生物炭 | 环丙沙星 | 99.01%±0.15% | SO | [ |
改性方式 | 改性材料 | 抗生素 | 降解率 | 主要自由基 | 文献 |
---|---|---|---|---|---|
纳米改性 | 纳米Fe0 | 磺胺甲唑 | 87.6% | ·OH(pH>8.5) | [ |
纳米Fe0 | 磺胺嘧啶 | 93% | — | [ | |
双金属体系 | Fe0/Ag | 左氧氟沙星 氯霉素 | 60% 91% | SO | [ |
纳米Fe0/Cu | 盐酸四环素 | 89% | SO | [ | |
预处理 | 超声 | 磺胺嘧啶 | 95.7% | SO | [ |
预磁化 | 磺胺嘧啶 | 49.3% | SO | [ | |
水热 | 氯霉素 | 70.89% | — | [ | |
材料负载 | 介孔炭负载纳米Fe0 | 四环素 | 92.1% | SO | [ |
生物炭负载Fe0/Ni | 诺氟沙星 | 90%以上 | SO | [ | |
硫化改性 | 硫化纳米Fe0 | 磺胺嘧啶 | 100% | — | [ |
硫化纳米Fe0/生物炭 | 环丙沙星 | 99.01%±0.15% | SO | [ |
不同离子 | 降解率 | 参考文献 |
---|---|---|
Cl- | 降解速率下降 | [ |
0.03mol/L Cl-使降解速率略有提高,浓度的进一步增加使降解率下降 | [ | |
Br- | 降解速率下降 | [ |
无显著影响 | [ | |
NO | 降解速率下降 | [ |
较弱抑制作用 | [ | |
HCO | 降解速率下降 | [ |
降解速率上升 | [ | |
无显著影响 | [ | |
SO | 降解速率下降 | [ |
降解率上升 | [ |
不同离子 | 降解率 | 参考文献 |
---|---|---|
Cl- | 降解速率下降 | [ |
0.03mol/L Cl-使降解速率略有提高,浓度的进一步增加使降解率下降 | [ | |
Br- | 降解速率下降 | [ |
无显著影响 | [ | |
NO | 降解速率下降 | [ |
较弱抑制作用 | [ | |
HCO | 降解速率下降 | [ |
降解速率上升 | [ | |
无显著影响 | [ | |
SO | 降解速率下降 | [ |
降解率上升 | [ |
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