Chemical Industry and Engineering Progress ›› 2022, Vol. 41 ›› Issue (4): 1873-1885.DOI: 10.16085/j.issn.1000-6613.2021-0732
• Industrial catalysis • Previous Articles Next Articles
LI Qinghui1,2(), SONG Huanling1, ZHAO Huahua1(), YANG Jian1, ZHAO Jun1, YAN Liang1, CHOU Lingjun1,3()
Received:
2021-04-08
Revised:
2021-07-21
Online:
2022-04-25
Published:
2022-04-23
Contact:
ZHAO Huahua,CHOU Lingjun
李庆慧1,2(), 宋焕玲1, 赵华华1(), 杨建1, 赵军1, 闫亮1, 丑凌军1,3()
通讯作者:
赵华华,丑凌军
作者简介:
李庆慧(1997—),女,硕士研究生,研究方向为多相催化。E-mail:基金资助:
CLC Number:
LI Qinghui, SONG Huanling, ZHAO Huahua, YANG Jian, ZHAO Jun, YAN Liang, CHOU Lingjun. Selective oxidation of light olefins to aldehydes catalyzed by molybdenum-bismuth composite metal oxides[J]. Chemical Industry and Engineering Progress, 2022, 41(4): 1873-1885.
李庆慧, 宋焕玲, 赵华华, 杨建, 赵军, 闫亮, 丑凌军. 钼铋复合金属氧化物催化低碳烯烃选择氧化制备醛类研究进展[J]. 化工进展, 2022, 41(4): 1873-1885.
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催化剂 | 反应温度/℃ | 反应空速/h-1 | 丙烯转化率% | 丙烯醛选择性% | 参考专利 |
---|---|---|---|---|---|
MoWBiFeCoNiKSi | 310 | 1400 | 97.5 | 85.2 | CN101402044A |
MoBiFeCoK | 320 | 5000 | 97.18 | 81.7 | CN1564709A |
MoWBiFeCoNiBKSi | 310 | 1565 | 98.2 | 81.6 | CN1093021A |
MoWBiFeCoKSi | 320 | 1800 | 97.6 | 90.2 | US3825600 |
MoBiFeCKSi | 320 | — | 99.1 | 88.8 | JP5293389 |
MoWBiFeCoNiK | 315 | 1200 | 98.5 | 82.5 | CN93103817 |
MoBiCoFeNiW | 305 | 850 | 98.1 | 85.6 | CN102992979A |
MoBiCoFeNiWCs | 320 | 1500 | 98.3 | 87.4 | CN102992979A |
MoBiCoFeNiKLa | 325 | 1200 | 98.3 | 87.7 | CN102992979A |
MoBiCoFeNiMgK | 310 | 1100 | 98.2 | 85.6 | CN102992979A |
MoBiCoFeNiKS | 367 | 1000 | 98.0 | 86.5 | CN102992979A |
催化剂 | 反应温度/℃ | 反应空速/h-1 | 丙烯转化率% | 丙烯醛选择性% | 参考专利 |
---|---|---|---|---|---|
MoWBiFeCoNiKSi | 310 | 1400 | 97.5 | 85.2 | CN101402044A |
MoBiFeCoK | 320 | 5000 | 97.18 | 81.7 | CN1564709A |
MoWBiFeCoNiBKSi | 310 | 1565 | 98.2 | 81.6 | CN1093021A |
MoWBiFeCoKSi | 320 | 1800 | 97.6 | 90.2 | US3825600 |
MoBiFeCKSi | 320 | — | 99.1 | 88.8 | JP5293389 |
MoWBiFeCoNiK | 315 | 1200 | 98.5 | 82.5 | CN93103817 |
MoBiCoFeNiW | 305 | 850 | 98.1 | 85.6 | CN102992979A |
MoBiCoFeNiWCs | 320 | 1500 | 98.3 | 87.4 | CN102992979A |
MoBiCoFeNiKLa | 325 | 1200 | 98.3 | 87.7 | CN102992979A |
MoBiCoFeNiMgK | 310 | 1100 | 98.2 | 85.6 | CN102992979A |
MoBiCoFeNiKS | 367 | 1000 | 98.0 | 86.5 | CN102992979A |
催化剂 | 反应温度/℃ | 反应空速/h-1 | 异丁烯转化率/% | 甲基丙烯醛选择性/% | 参考专利 |
---|---|---|---|---|---|
MoBiFeCoCe | 300 | 3600 | 98.7 | 97.1 | US5138100 |
MoBiFeCoPr | 340 | 3600 | 99.0 | 94.0 | US5138100 |
MoBiFeCoEu | 360 | 3600 | 99.1 | 93.0 | US5138100 |
MoBiFeZnCsSb | 330 | 800 | 95.4 | 87.7 | WO9926912 |
MoBiFeWCoCsSiZr | 330 | 1600 | 98.5 | 88.2 | EP685260 |
MoBiFeNiWCoMgZnBSbCsSi | 365 | — | 97.1 | 88.2 | JP11179206 |
MoBiFeCoCs | — | 750 | 99.5 | 83.3 | JP2000288396 |
MoBiFeNiCoZnGeTeCs | 340 | 800 | 97.6 | 88.2 | JP2000237592 |
MoWBiFeCoNiKSi | 310 | 1800 | 98.5 | 95.1 | JP2000325795 |
MoBiFeNiWCoMgZnBSbCs | 365 | 1000 | 95.5 | 88.8 | US5532199 |
MoBiFeCoMnPbPZrCsNa | 350 | 800 | 98.7 | 86.0 | US5856259 |
催化剂 | 反应温度/℃ | 反应空速/h-1 | 异丁烯转化率/% | 甲基丙烯醛选择性/% | 参考专利 |
---|---|---|---|---|---|
MoBiFeCoCe | 300 | 3600 | 98.7 | 97.1 | US5138100 |
MoBiFeCoPr | 340 | 3600 | 99.0 | 94.0 | US5138100 |
MoBiFeCoEu | 360 | 3600 | 99.1 | 93.0 | US5138100 |
MoBiFeZnCsSb | 330 | 800 | 95.4 | 87.7 | WO9926912 |
MoBiFeWCoCsSiZr | 330 | 1600 | 98.5 | 88.2 | EP685260 |
MoBiFeNiWCoMgZnBSbCsSi | 365 | — | 97.1 | 88.2 | JP11179206 |
MoBiFeCoCs | — | 750 | 99.5 | 83.3 | JP2000288396 |
MoBiFeNiCoZnGeTeCs | 340 | 800 | 97.6 | 88.2 | JP2000237592 |
MoWBiFeCoNiKSi | 310 | 1800 | 98.5 | 95.1 | JP2000325795 |
MoBiFeNiWCoMgZnBSbCs | 365 | 1000 | 95.5 | 88.8 | US5532199 |
MoBiFeCoMnPbPZrCsNa | 350 | 800 | 98.7 | 86.0 | US5856259 |
催化剂 | 比表面积/m2·g-1 |
---|---|
纯α-Bi2Mo3O12 | 2 |
共沉淀法BiMoO+TiO2 | 40 |
浸渍法BiMoO+TiO2 | 39 |
溶胶-凝胶法BiMoO+TiO2 | 108 |
催化剂 | 比表面积/m2·g-1 |
---|---|
纯α-Bi2Mo3O12 | 2 |
共沉淀法BiMoO+TiO2 | 40 |
浸渍法BiMoO+TiO2 | 39 |
溶胶-凝胶法BiMoO+TiO2 | 108 |
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