Chemical Industry and Engineering Progress ›› 2019, Vol. 38 ›› Issue (03): 1269-1282.DOI: 10.16085/j.issn.1000-6613.2018-0984
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Lungang CHEN(),Xinghua ZHANG,Qi ZHANG,Chenguang WANG,Longlong MA()
Received:
2018-05-14
Revised:
2018-06-05
Online:
2019-03-05
Published:
2019-03-05
Contact:
Longlong MA
通讯作者:
马隆龙
作者简介:
基金资助:
CLC Number:
Lungang CHEN,Xinghua ZHANG,Qi ZHANG,Chenguang WANG,Longlong MA. Progress in aviation biofuel technology by catalysis synthesis of platform molecules from lignocelluloses depolymerization[J]. Chemical Industry and Engineering Progress, 2019, 38(03): 1269-1282.
陈伦刚,张兴华,张琦,王晨光,马隆龙. 木质纤维素解聚平台分子催化合成航油技术的进展[J]. 化工进展, 2019, 38(03): 1269-1282.
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URL: https://hgjz.cip.com.cn/EN/10.16085/j.issn.1000-6613.2018-0984
序号 | 技术路径 | 平台分子原料要求 | 技术路径优势 | 技术路径缺点 |
---|---|---|---|---|
1 | 羟烷基化途径 | 纯度、浓度和杂质要求高 | 碳利用率高、目标烃类产物选择性高、燃料分子结构调控性强 | 工艺流程长、受限于来源于半纤维素的2-甲基糠醛、平台分子分离提纯导致能耗高、损耗大 |
2 | 羟醛缩合途径 | 纯度、浓度和杂质要求不高 | 碳利用率高、目标烃类产物选择性高、燃料分子结构调控性强、纤维素和半纤维素解聚的平台分子可同步利用 | 工艺流程较长、酸碱消耗大 |
3 | 水相重整途径 | 纯度、浓度和杂质要求不高 | 工艺流程短、纤维素和半纤维素来的平台分子可同步利用 | 碳利用率低、目标烃类产物选择性低、燃料分子结构调控性差 |
4 | 烯烃聚合途径 | 纯度、浓度和杂质要求高 | 烯烃聚合后的加氢反应条件温和易实现 | 工艺流程长、碳利用率较低、目标烃类产物选择性较低、燃料分子结构调控性较差、对烯烃的纯度要求高 |
序号 | 技术路径 | 平台分子原料要求 | 技术路径优势 | 技术路径缺点 |
---|---|---|---|---|
1 | 羟烷基化途径 | 纯度、浓度和杂质要求高 | 碳利用率高、目标烃类产物选择性高、燃料分子结构调控性强 | 工艺流程长、受限于来源于半纤维素的2-甲基糠醛、平台分子分离提纯导致能耗高、损耗大 |
2 | 羟醛缩合途径 | 纯度、浓度和杂质要求不高 | 碳利用率高、目标烃类产物选择性高、燃料分子结构调控性强、纤维素和半纤维素解聚的平台分子可同步利用 | 工艺流程较长、酸碱消耗大 |
3 | 水相重整途径 | 纯度、浓度和杂质要求不高 | 工艺流程短、纤维素和半纤维素来的平台分子可同步利用 | 碳利用率低、目标烃类产物选择性低、燃料分子结构调控性差 |
4 | 烯烃聚合途径 | 纯度、浓度和杂质要求高 | 烯烃聚合后的加氢反应条件温和易实现 | 工艺流程长、碳利用率较低、目标烃类产物选择性较低、燃料分子结构调控性较差、对烯烃的纯度要求高 |
序号 | 主要成分 | 分子结构 | 碳数 | 相对丰度/% |
---|---|---|---|---|
1 | 3-甲基庚烷 | 8 | 4.03 | |
2 | 正辛烷 | 8 | 4.64 | |
3 | 4-甲基辛烷 | 9 | 3.49 | |
4 | 3-甲基辛烷 | 9 | 3.59 | |
5 | 正壬烷 | 9 | 3.41 | |
6 | 4-甲基壬烷 | 10 | 2.81 | |
7 | 正癸烷 | 10 | 2.10 | |
8 | 丁基-环己烷 | 10 | 0.71 | |
9 | 5-甲基癸烷 | 11 | 2.64 | |
10 | 4-甲基癸烷 | 11 | 2.74 | |
11 | 正十一烷 | 11 | 1.97 | |
12 | 5-甲基十一烷 | 12 | 20.04 | |
13 | 正十二烷 | 12 | 3.03 | |
14 | 正十三烷 | 13 | 6.58 | |
15 | 5-甲基十二烷 | 13 | 24.19 | |
16 | 1,1,3,5-四甲基环己烷 | 10 | 1.28 | |
17 | 1,2-二丁基环戊烷 | 14 | 1.53 | |
18 | 6-甲基十三烷 | 14 | 8.11 | |
19 | 1-甲基-4-异丙基环己烷 | 10 | 2.86 | |
20 | 2,7-二甲基萘 | 12 | 0.15 | |
21 | 1-甲基-3-异丙基环己烷 | 10 | 0.09 |
序号 | 主要成分 | 分子结构 | 碳数 | 相对丰度/% |
---|---|---|---|---|
1 | 3-甲基庚烷 | 8 | 4.03 | |
2 | 正辛烷 | 8 | 4.64 | |
3 | 4-甲基辛烷 | 9 | 3.49 | |
4 | 3-甲基辛烷 | 9 | 3.59 | |
5 | 正壬烷 | 9 | 3.41 | |
6 | 4-甲基壬烷 | 10 | 2.81 | |
7 | 正癸烷 | 10 | 2.10 | |
8 | 丁基-环己烷 | 10 | 0.71 | |
9 | 5-甲基癸烷 | 11 | 2.64 | |
10 | 4-甲基癸烷 | 11 | 2.74 | |
11 | 正十一烷 | 11 | 1.97 | |
12 | 5-甲基十一烷 | 12 | 20.04 | |
13 | 正十二烷 | 12 | 3.03 | |
14 | 正十三烷 | 13 | 6.58 | |
15 | 5-甲基十二烷 | 13 | 24.19 | |
16 | 1,1,3,5-四甲基环己烷 | 10 | 1.28 | |
17 | 1,2-二丁基环戊烷 | 14 | 1.53 | |
18 | 6-甲基十三烷 | 14 | 8.11 | |
19 | 1-甲基-4-异丙基环己烷 | 10 | 2.86 | |
20 | 2,7-二甲基萘 | 12 | 0.15 | |
21 | 1-甲基-3-异丙基环己烷 | 10 | 0.09 |
样品 | 各元素质量分数/% | 热值 /MJ·kg-1 | ||
---|---|---|---|---|
C | H | O | ||
玉米秸秆 | 45.76% | 6.22% | 47.79% | 16.1 |
缩合产物 | 62.53% | 4.75% | 32.72% | 30.8 |
加氢后的 | 59.66% | 8.73% | 31.43% | 32.7 |
加氢脱氧后的 | 81.39% | 14.07% | 4.09% | 41.7 |
加氢精制后的 | 84.15% | 15.24% | 0.37% | 45.5 |
样品 | 各元素质量分数/% | 热值 /MJ·kg-1 | ||
---|---|---|---|---|
C | H | O | ||
玉米秸秆 | 45.76% | 6.22% | 47.79% | 16.1 |
缩合产物 | 62.53% | 4.75% | 32.72% | 30.8 |
加氢后的 | 59.66% | 8.73% | 31.43% | 32.7 |
加氢脱氧后的 | 81.39% | 14.07% | 4.09% | 41.7 |
加氢精制后的 | 84.15% | 15.24% | 0.37% | 45.5 |
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