Chemical Industry and Engineering Progress ›› 2022, Vol. 41 ›› Issue (10): 5259-5271.DOI: 10.16085/j.issn.1000-6613.2021-2632
• Energy processes and technology • Previous Articles Next Articles
ZHANG Xuemin1,2,3(), ZHANG Shanling1,2,3, LI Pengyu1,2,3, HUANG Tingting1,2,3, YIN Shaoqi1,2,3, LI Jinping1,2,3, WANG Yingmei1,2,4
Received:
2021-12-27
Revised:
2022-02-15
Online:
2022-10-21
Published:
2022-10-20
Contact:
ZHANG Xuemin
张学民1,2,3(), 张山岭1,2,3, 李鹏宇1,2,3, 黄婷婷1,2,3, 尹绍奇1,2,3, 李金平1,2,3, 王英梅1,2,4
通讯作者:
张学民
作者简介:
张学民(1987—),男,博士,副教授,硕士生导师,主要从事气体水合物生成与分解动力学方面的研究。E-mail:zxm2010lut@163.com。
基金资助:
CLC Number:
ZHANG Xuemin, ZHANG Shanling, LI Pengyu, HUANG Tingting, YIN Shaoqi, LI Jinping, WANG Yingmei. Research progress on influencing factors and strengthening mechanism of CO2-CH4 hydrate replacement in porous media system[J]. Chemical Industry and Engineering Progress, 2022, 41(10): 5259-5271.
张学民, 张山岭, 李鹏宇, 黄婷婷, 尹绍奇, 李金平, 王英梅. 多孔介质中CO2-CH4水合物置换的影响因素及强化机理研究进展[J]. 化工进展, 2022, 41(10): 5259-5271.
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URL: https://hgjz.cip.com.cn/EN/10.16085/j.issn.1000-6613.2021-2632
气体名称 | 优点 | 缺点 |
---|---|---|
N2 | 价格低廉 使用安全 | 过量会抑制CO2水合物生成 分离麻烦、成本高 |
H2 | 置换效果更好 少量H2可以促进CO2水合物生成 | 成本昂贵 过量会抑制CO2水合物生成存在安全隐患 |
气体名称 | 优点 | 缺点 |
---|---|---|
N2 | 价格低廉 使用安全 | 过量会抑制CO2水合物生成 分离麻烦、成本高 |
H2 | 置换效果更好 少量H2可以促进CO2水合物生成 | 成本昂贵 过量会抑制CO2水合物生成存在安全隐患 |
CH4回收率 /% | 置换时初始压力 /MPa | 热刺激方式 | 研究者 |
---|---|---|---|
68.8 | 3.3 | 加热功率为100W | Tupsakhare等[ |
49.42 | 8.03 | 每两小时加热15min(共加热三次) | Ouyang等[ |
64.6 | 2.13 | 温度从273.65K提升到279.15K并维持2h | Zhang等[ |
75~93 | 2 | 温度升到289.15K并保持200min | Yang等[ |
82.2 | 3 | 温度设置成275.65K并保持18h | Stanwix等[ |
60 | 3 | 温度在271.15~278.15K循环 | Tupsakhare等[ |
44 | 7.8 | 升高温度直至观察到分解时刻 | Gambelli等[ |
CH4回收率 /% | 置换时初始压力 /MPa | 热刺激方式 | 研究者 |
---|---|---|---|
68.8 | 3.3 | 加热功率为100W | Tupsakhare等[ |
49.42 | 8.03 | 每两小时加热15min(共加热三次) | Ouyang等[ |
64.6 | 2.13 | 温度从273.65K提升到279.15K并维持2h | Zhang等[ |
75~93 | 2 | 温度升到289.15K并保持200min | Yang等[ |
82.2 | 3 | 温度设置成275.65K并保持18h | Stanwix等[ |
60 | 3 | 温度在271.15~278.15K循环 | Tupsakhare等[ |
44 | 7.8 | 升高温度直至观察到分解时刻 | Gambelli等[ |
CH4回收率 /% | 置换时初始温度 /K | 压力或减压方式 | 研究者 |
---|---|---|---|
32.66 | 273.65 | 每次减压时压力从2.92MPa降到1.74MPa并维持30min(共减压三次) | Sun等[ |
63.3 | 274.15 | 通过减压使水合物分解比为20%时再进行置换 | Lee等[ |
71 | 274.15 | CO2气体分压为1.8MPa | Ding等[ |
66 | 276.2 | 压力降至2MPa直至置换反应结束 | Sun等[ |
85.3~89.1 | 279.15 | 通过多级减压将压力从6MPa降至3MPa | Gao等[ |
49 | 277.2 | 实验压力为3.5MPa | Liu等[ |
31 | 276.15 | CO2气体分压为4.5MPa | Xu等[ |
CH4回收率 /% | 置换时初始温度 /K | 压力或减压方式 | 研究者 |
---|---|---|---|
32.66 | 273.65 | 每次减压时压力从2.92MPa降到1.74MPa并维持30min(共减压三次) | Sun等[ |
63.3 | 274.15 | 通过减压使水合物分解比为20%时再进行置换 | Lee等[ |
71 | 274.15 | CO2气体分压为1.8MPa | Ding等[ |
66 | 276.2 | 压力降至2MPa直至置换反应结束 | Sun等[ |
85.3~89.1 | 279.15 | 通过多级减压将压力从6MPa降至3MPa | Gao等[ |
49 | 277.2 | 实验压力为3.5MPa | Liu等[ |
31 | 276.15 | CO2气体分压为4.5MPa | Xu等[ |
方法 | 温度/K | 压力/MPa | 反应时间/h | CH4回收率/% | 研究者 |
---|---|---|---|---|---|
气态CO2 | 273 | 3.36 | 100 | 20 | Ota等[ |
气态CO2 | 272.2 | 3.6/4.0/4.5 | 150 | 8.63/10.89/13.2 | Zhang等[ |
气态CO2 | 275 | 2.91/2.93 | 225/200 | 23/6 | Li等[ |
气态CO2 | 274 | 4.5 | 34 | 35 | Ryou等[ |
液态CO2 | 273.2 | 4 | 700 | 26.4 | Wang等[ |
液态CO2 | 282.2 | 6 | 288 | 45 | Li等[ |
液态CO2 | 275 | 9 | 80 | 40.2 | Lee等[ |
CO2乳化液 | 281.2 | 5 | 96 | 27.1 | Zhou等[ |
CO2+N2(25∶75) | 274.2 | 10 | 280 | 25 | Pan等[ |
CO2+N2(20∶80) | 274 | 17 | 72 | 39 | Choi等[ |
CO2+N2(60∶40) | 274 | 4.5 | 192 | 73.42 | Xu等[ |
CO2+N2(21∶79) | 285.2 | 12/15 | 200 | 86/75 | Li等[ |
CO2+H2(60∶40) | 274.15 | 4.5 | 192 | 70.21 | Ding等[ |
CO2+H2(18∶82) | 275.65 | 5 | 300 | 70 | Wang等[ |
CO2+H2(40∶60) | 274 | 4.5 | 192 | 78.02 | Xu等[ |
CO2+H2(56∶44) | 276.12~276.23 | 3.70~3.80 | 4 | 61~75 | Sun等[ |
CO2+H2(43∶57) | 276 | 3.67 | 320 | 61 | Sun等[ |
CO2+H2(0∶100) | 276 | 3.67 | 320 | 63 | Sun等[ |
CO2+CH3OH | 274.41 | 3.3 | 56.62 | 92 | Khlebnikov等[ |
CO2+Rhamnolipid(鼠李糖脂) | 276.15 | 3.1 | 92 | 18.02 | Heydari等[ |
CO2+TMACl(四甲基氯化铵) | 274.15 | 6 | 24 | 83 | Moujdin等[ |
方法 | 温度/K | 压力/MPa | 反应时间/h | CH4回收率/% | 研究者 |
---|---|---|---|---|---|
气态CO2 | 273 | 3.36 | 100 | 20 | Ota等[ |
气态CO2 | 272.2 | 3.6/4.0/4.5 | 150 | 8.63/10.89/13.2 | Zhang等[ |
气态CO2 | 275 | 2.91/2.93 | 225/200 | 23/6 | Li等[ |
气态CO2 | 274 | 4.5 | 34 | 35 | Ryou等[ |
液态CO2 | 273.2 | 4 | 700 | 26.4 | Wang等[ |
液态CO2 | 282.2 | 6 | 288 | 45 | Li等[ |
液态CO2 | 275 | 9 | 80 | 40.2 | Lee等[ |
CO2乳化液 | 281.2 | 5 | 96 | 27.1 | Zhou等[ |
CO2+N2(25∶75) | 274.2 | 10 | 280 | 25 | Pan等[ |
CO2+N2(20∶80) | 274 | 17 | 72 | 39 | Choi等[ |
CO2+N2(60∶40) | 274 | 4.5 | 192 | 73.42 | Xu等[ |
CO2+N2(21∶79) | 285.2 | 12/15 | 200 | 86/75 | Li等[ |
CO2+H2(60∶40) | 274.15 | 4.5 | 192 | 70.21 | Ding等[ |
CO2+H2(18∶82) | 275.65 | 5 | 300 | 70 | Wang等[ |
CO2+H2(40∶60) | 274 | 4.5 | 192 | 78.02 | Xu等[ |
CO2+H2(56∶44) | 276.12~276.23 | 3.70~3.80 | 4 | 61~75 | Sun等[ |
CO2+H2(43∶57) | 276 | 3.67 | 320 | 61 | Sun等[ |
CO2+H2(0∶100) | 276 | 3.67 | 320 | 63 | Sun等[ |
CO2+CH3OH | 274.41 | 3.3 | 56.62 | 92 | Khlebnikov等[ |
CO2+Rhamnolipid(鼠李糖脂) | 276.15 | 3.1 | 92 | 18.02 | Heydari等[ |
CO2+TMACl(四甲基氯化铵) | 274.15 | 6 | 24 | 83 | Moujdin等[ |
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