Chemical Industry and Engineering Progress ›› 2020, Vol. 39 ›› Issue (S2): 185-195.DOI: 10.16085/j.issn.1000-6613.2020-1266
• Industrial catalysis • Previous Articles Next Articles
Weiyue WANG1, Peipei ZHAO1, Lingyun JIN2, Bingheng CEN1, Jian CHEN1(), Mengfei LUO1
Received:
2020-07-06
Online:
2020-11-17
Published:
2020-11-20
Contact:
Jian CHEN
王炜月1, 赵培培1, 金凌云2, 岑丙横1, 陈建1(), 罗孟飞1
通讯作者:
陈建
作者简介:
王炜月(1997—),女,硕士研究生,研究方向为环境催化。
基金资助:
CLC Number:
Weiyue WANG, Peipei ZHAO, Lingyun JIN, Bingheng CEN, Jian CHEN, Mengfei LUO. Recent advances in catalysts for volatile organic compounds combustion[J]. Chemical Industry and Engineering Progress, 2020, 39(S2): 185-195.
王炜月, 赵培培, 金凌云, 岑丙横, 陈建, 罗孟飞. 挥发性有机物燃烧催化剂的研究进展[J]. 化工进展, 2020, 39(S2): 185-195.
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URL: https://hgjz.cip.com.cn/EN/10.16085/j.issn.1000-6613.2020-1266
催化剂 | 转化率①/% | Pt0/(Pt0+Pt2+) | 质量比速率 /μmol·s-1·g-1 | |
---|---|---|---|---|
新鲜催化剂 | 用过催化剂② | |||
Pt/Al2O3 | 11.4 | 0.15 | 0.51 | 11.3 |
Pt-2Nb/Al2O3 | 17.6 | 0.34 | 0.65 | 17.5 |
Pt-6Nb/Al2O3 | 48.1 | 0.47 | 0.70 | 47.7 |
Pt-10Nb/Al2O3 | 62.3 | 0.66 | 0.71 | 61.8 |
Pt-15Nb/Al2O3 | 55.9 | 0.87 | 0.91 | 55.5 |
10Nb/Al2O3 | 0 | — | — | — |
Pt-10Nb/Al2O3-R | 69.8 | 0.86 | 0.86 | 69.2 |
催化剂 | 转化率①/% | Pt0/(Pt0+Pt2+) | 质量比速率 /μmol·s-1·g-1 | |
---|---|---|---|---|
新鲜催化剂 | 用过催化剂② | |||
Pt/Al2O3 | 11.4 | 0.15 | 0.51 | 11.3 |
Pt-2Nb/Al2O3 | 17.6 | 0.34 | 0.65 | 17.5 |
Pt-6Nb/Al2O3 | 48.1 | 0.47 | 0.70 | 47.7 |
Pt-10Nb/Al2O3 | 62.3 | 0.66 | 0.71 | 61.8 |
Pt-15Nb/Al2O3 | 55.9 | 0.87 | 0.91 | 55.5 |
10Nb/Al2O3 | 0 | — | — | — |
Pt-10Nb/Al2O3-R | 69.8 | 0.86 | 0.86 | 69.2 |
催化剂 | 选择性/% | |||||||||
---|---|---|---|---|---|---|---|---|---|---|
T98 | 300℃ | 340℃ | 400℃ | 420℃ | ||||||
CO | N2 | CO | N2 | CO | N2 | CO | N2 | CO | N2 | |
4MnOx/ZSM-5(18) | 7.2 | 100 | 4.4 | 100 | 0 | 100 | 0 | 100 | 0 | 100 |
12MnOx/ZSM-5(18) | 2.0 | 100 | 0 | 100 | 0 | 100 | 0 | 99.2 | 0 | 98.5 |
20MnOx/ZSM-5(18) | 1.2 | 100 | 0 | 100 | 0 | 100 | 0 | 98.5 | 0 | 95.5 |
4MnOx/ZSM-5(360) | 2.8 | 100 | 2.0 | 100 | 0 | 99.2 | 0 | 91.3 | 0 | 84.3 |
12MnOx/ZSM-5(360) | 1.8 | 100 | 0 | 100 | 0 | 93.2 | 0 | 72.6 | 0 | 62.7 |
20MnOx/ZSM-5(360) | 0.8 | 100 | 0 | 97.7 | 0 | 89.0 | 0 | 69.1 | 0 | 58.3 |
12MnOx/SiO2 | 6.0 | 90.4 | 2.6 | 67.4 | 0 | 44.7 | 0 | 28.5 | 0 | 22.1 |
催化剂 | 选择性/% | |||||||||
---|---|---|---|---|---|---|---|---|---|---|
T98 | 300℃ | 340℃ | 400℃ | 420℃ | ||||||
CO | N2 | CO | N2 | CO | N2 | CO | N2 | CO | N2 | |
4MnOx/ZSM-5(18) | 7.2 | 100 | 4.4 | 100 | 0 | 100 | 0 | 100 | 0 | 100 |
12MnOx/ZSM-5(18) | 2.0 | 100 | 0 | 100 | 0 | 100 | 0 | 99.2 | 0 | 98.5 |
20MnOx/ZSM-5(18) | 1.2 | 100 | 0 | 100 | 0 | 100 | 0 | 98.5 | 0 | 95.5 |
4MnOx/ZSM-5(360) | 2.8 | 100 | 2.0 | 100 | 0 | 99.2 | 0 | 91.3 | 0 | 84.3 |
12MnOx/ZSM-5(360) | 1.8 | 100 | 0 | 100 | 0 | 93.2 | 0 | 72.6 | 0 | 62.7 |
20MnOx/ZSM-5(360) | 0.8 | 100 | 0 | 97.7 | 0 | 89.0 | 0 | 69.1 | 0 | 58.3 |
12MnOx/SiO2 | 6.0 | 90.4 | 2.6 | 67.4 | 0 | 44.7 | 0 | 28.5 | 0 | 22.1 |
催化剂 | T98/℃ | 选择性/% | |||||
---|---|---|---|---|---|---|---|
T98 | 300℃ | 400℃ | |||||
CO | N2 | CO | N2 | CO | N2 | ||
2CuO/ZSM-5-18 | 300 | 6.4 | 100 | 6.4 | 100 | 0 | 98.5 |
4CuO/ZSM-5-18 | 280 | 2.8 | 100 | 0.2 | 100 | 0 | 96.2 |
6CuO/ZSM-5-18 | 240 | 2.8 | 100 | 0 | 100 | 0 | 95.5 |
10CuO/ZSM-5-18 | 240 | 2.0 | 100 | 0 | 100 | 0 | 94.7 |
14CuO/ZSM-5-18 | 240 | 2.0 | 100 | 0 | 100 | 0 | 94.0 |
催化剂 | T98/℃ | 选择性/% | |||||
---|---|---|---|---|---|---|---|
T98 | 300℃ | 400℃ | |||||
CO | N2 | CO | N2 | CO | N2 | ||
2CuO/ZSM-5-18 | 300 | 6.4 | 100 | 6.4 | 100 | 0 | 98.5 |
4CuO/ZSM-5-18 | 280 | 2.8 | 100 | 0.2 | 100 | 0 | 96.2 |
6CuO/ZSM-5-18 | 240 | 2.8 | 100 | 0 | 100 | 0 | 95.5 |
10CuO/ZSM-5-18 | 240 | 2.0 | 100 | 0 | 100 | 0 | 94.7 |
14CuO/ZSM-5-18 | 240 | 2.0 | 100 | 0 | 100 | 0 | 94.0 |
VOCs名称 | 最弱的CH键/kJ·mol-1 | 极性 | Cu0.15Mn0.3Ce0.55/CH | 商品Pd/Al2O3 | ||
---|---|---|---|---|---|---|
T50/℃ | T95/℃ | T50/℃ | T95/℃ | |||
苯 | 426.2 | 0 | 225 | 250 | 245 | 270 |
甲苯 | 370.3 | 0.45 | 235 | 240 | 225 | 235 |
邻二甲苯 | — | 0.33 | 250 | 280 | 215 | 225 |
己烷 | 395.0 | 0 | 190 | 210 | 330 | 345 |
环己烷 | 399.0 | 0 | 200 | 240 | 330 | 325 |
乙醇 | 396.6 | 1.69 | 160 | 175 | 220 | 245 |
乙醛 | 394.3 | 2.71 | 170 | 190 | 240 | 250 |
乙酸乙酯 | — | 1.78 | 180 | 190 | 260 | 270 |
甲基丙烯酸甲酯 | — | 1.68 | 195 | 210 | 210 | 220 |
丙酮 | 411.5 | 2.77 | 185 | 195 | 230 | 250 |
VOCs名称 | 最弱的CH键/kJ·mol-1 | 极性 | Cu0.15Mn0.3Ce0.55/CH | 商品Pd/Al2O3 | ||
---|---|---|---|---|---|---|
T50/℃ | T95/℃ | T50/℃ | T95/℃ | |||
苯 | 426.2 | 0 | 225 | 250 | 245 | 270 |
甲苯 | 370.3 | 0.45 | 235 | 240 | 225 | 235 |
邻二甲苯 | — | 0.33 | 250 | 280 | 215 | 225 |
己烷 | 395.0 | 0 | 190 | 210 | 330 | 345 |
环己烷 | 399.0 | 0 | 200 | 240 | 330 | 325 |
乙醇 | 396.6 | 1.69 | 160 | 175 | 220 | 245 |
乙醛 | 394.3 | 2.71 | 170 | 190 | 240 | 250 |
乙酸乙酯 | — | 1.78 | 180 | 190 | 260 | 270 |
甲基丙烯酸甲酯 | — | 1.68 | 195 | 210 | 210 | 220 |
丙酮 | 411.5 | 2.77 | 185 | 195 | 230 | 250 |
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