Chemical Industry and Engineering Progress ›› 2021, Vol. 40 ›› Issue (5): 2784-2801.DOI: 10.16085/j.issn.1000-6613.2020-1274
• Resources and environmental engineering • Previous Articles Next Articles
SUN Yilei(), MA Yue, LI Shuyuan, YUE Changtao()
Received:
2020-07-06
Online:
2021-05-24
Published:
2021-05-06
Contact:
YUE Changtao
通讯作者:
岳长涛
作者简介:
孙艺蕾(1996—),女,硕士研究生,研究方向为高密度聚乙烯热解生产α-烯烃。E-mail:CLC Number:
SUN Yilei, MA Yue, LI Shuyuan, YUE Changtao. Research progress in the pyrolysis and catalytic pyrolysis of waste polyolefin plastics[J]. Chemical Industry and Engineering Progress, 2021, 40(5): 2784-2801.
孙艺蕾, 马跃, 李术元, 岳长涛. 聚烯烃塑料的热解和催化热解研究进展[J]. 化工进展, 2021, 40(5): 2784-2801.
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塑料名称 | 反应器类型 | 热解温度/℃ | 停留时间/s | 产物(质量分数)/% | |||
---|---|---|---|---|---|---|---|
蜡 | 轻质芳烃 | 低碳烯烃 | 苯乙烯 | ||||
HDPE[ LDPE[ HDPE[ HDPE[ PE/PP19] HDPE[ HDPE[ PP[ HDPE[ HDPE[ HDPE[ LLDPE[ PS[ | 锥形喷射床 流化床 流化床 流化床 锥形喷射床 流化砂床 流化床 流化床 流化床 流化床 锥形喷射床+多管 固定床 锥形喷射床 | 500~700 500~700 650 640~645 450 700~800 780 668~746 604~800 700~800 500、900~950 450、900 450~500 | — 15 0.8~1.0 0.82~0.99 — — 0.7~1.6 — — 0.7~2.27 0.016 1.3 — | 70~12 45.3~4.0 51.9~25.3 78.9~79.7 80/92 — 0.2~0 2.5~0 — 30~12 — — — | — — — — — 2.42~3.24 3.8~5.9 18~52 0.82~3.08 — — — 3.06~5.26 | 1.5~37 6.92~53.08 — — — 20.63~26.82 — 28~18.5 13.92~37.87 47.2~62.5 77~55 46.5 0.32~1.23 | — — — — — 0 1.7~0.7 0.8~2.8 — — — — 50.8~70.6 |
塑料名称 | 反应器类型 | 热解温度/℃ | 停留时间/s | 产物(质量分数)/% | |||
---|---|---|---|---|---|---|---|
蜡 | 轻质芳烃 | 低碳烯烃 | 苯乙烯 | ||||
HDPE[ LDPE[ HDPE[ HDPE[ PE/PP19] HDPE[ HDPE[ PP[ HDPE[ HDPE[ HDPE[ LLDPE[ PS[ | 锥形喷射床 流化床 流化床 流化床 锥形喷射床 流化砂床 流化床 流化床 流化床 流化床 锥形喷射床+多管 固定床 锥形喷射床 | 500~700 500~700 650 640~645 450 700~800 780 668~746 604~800 700~800 500、900~950 450、900 450~500 | — 15 0.8~1.0 0.82~0.99 — — 0.7~1.6 — — 0.7~2.27 0.016 1.3 — | 70~12 45.3~4.0 51.9~25.3 78.9~79.7 80/92 — 0.2~0 2.5~0 — 30~12 — — — | — — — — — 2.42~3.24 3.8~5.9 18~52 0.82~3.08 — — — 3.06~5.26 | 1.5~37 6.92~53.08 — — — 20.63~26.82 — 28~18.5 13.92~37.87 47.2~62.5 77~55 46.5 0.32~1.23 | — — — — — 0 1.7~0.7 0.8~2.8 — — — — 50.8~70.6 |
塑料名称 | 反应器类型 | 催化剂 | 反应温度/℃ | 产物(质量分数)/% | |||
---|---|---|---|---|---|---|---|
低碳烯烃 | 汽油 | 芳烃 | 苯乙烯 | ||||
HDPE[ HDPE[ LDPE[ HDPE[ HDPE[ HDPE[ HDPE[ PP[ PP[ PS[ PS[ PS[ PS[ PS[ PS[ PS[ PS[ PS[ | 锥形喷射床 锥形喷射床+固定床 固定床 固定床 锥形喷射床 锥形喷射床 固定床 流化床 流化床 固定床 固定床 固定床 固定床 固定床 固定床 固定床 固定床 固定床 | HZSM-5 HZSM-5(Si/Al=30) 酸改性的丝光沸石 FCC Hβ HY Al-MCM-41 MCM-41/SAHA/HUSY HZSM-5/HMOR Hβ AmY HY USY(Si/Al=5.3) Fe-MCM-41 HY/SBA-15 BaO Zn K2O/Si-MCM-41 | 450~500 500 400~500 430 500 500 450 360 360 400 400 400 650 450 650 350 450 400 | 56.4~54.1 58 0 50 30~40 17.97 38 26/24/28 49 — — — — — — — — — | 28.3~29.4 15.2 5.27~13.87 — 45~55 68.65 56 60.56/63.65/51.83 25.54/27.95 — — — — — — — — — | 6.77~4.23 11 0~1.62 — 5~10 24.10 4 0.16/0.25/0.93 1.82/0.48 55.74苯/3.5乙苯 49.08苯/19.2乙苯 33.5苯/34.79乙苯 31.1苯/34.0乙苯 7.5甲苯/22.0乙苯 58.4苯/10.2乙苯 1.6甲苯/0.2乙苯 2.5甲苯/1.16乙苯 — | — — 0 — 0 0 — — — 2.05 0 0 2.5 17 4.36 76.4 47.96 69.02 |
塑料名称 | 反应器类型 | 催化剂 | 反应温度/℃ | 产物(质量分数)/% | |||
---|---|---|---|---|---|---|---|
低碳烯烃 | 汽油 | 芳烃 | 苯乙烯 | ||||
HDPE[ HDPE[ LDPE[ HDPE[ HDPE[ HDPE[ HDPE[ PP[ PP[ PS[ PS[ PS[ PS[ PS[ PS[ PS[ PS[ PS[ | 锥形喷射床 锥形喷射床+固定床 固定床 固定床 锥形喷射床 锥形喷射床 固定床 流化床 流化床 固定床 固定床 固定床 固定床 固定床 固定床 固定床 固定床 固定床 | HZSM-5 HZSM-5(Si/Al=30) 酸改性的丝光沸石 FCC Hβ HY Al-MCM-41 MCM-41/SAHA/HUSY HZSM-5/HMOR Hβ AmY HY USY(Si/Al=5.3) Fe-MCM-41 HY/SBA-15 BaO Zn K2O/Si-MCM-41 | 450~500 500 400~500 430 500 500 450 360 360 400 400 400 650 450 650 350 450 400 | 56.4~54.1 58 0 50 30~40 17.97 38 26/24/28 49 — — — — — — — — — | 28.3~29.4 15.2 5.27~13.87 — 45~55 68.65 56 60.56/63.65/51.83 25.54/27.95 — — — — — — — — — | 6.77~4.23 11 0~1.62 — 5~10 24.10 4 0.16/0.25/0.93 1.82/0.48 55.74苯/3.5乙苯 49.08苯/19.2乙苯 33.5苯/34.79乙苯 31.1苯/34.0乙苯 7.5甲苯/22.0乙苯 58.4苯/10.2乙苯 1.6甲苯/0.2乙苯 2.5甲苯/1.16乙苯 — | — — 0 — 0 0 — — — 2.05 0 0 2.5 17 4.36 76.4 47.96 69.02 |
原料 | 脱氯方法 | 反应温度/℃ | 停留时间/min | 催化剂 | 吸附剂 | 油质量分数/% | 油中氯质量分数/% |
---|---|---|---|---|---|---|---|
PVC[ PVC[ PE\PP\PS\PVC\PET[ PE\PP\PS\PVC\PET[ PP\PVC[ PE\PP\PS\PVC[ | 热解 逐步热解 逐步热解 分步催化热解 催化热解 吸附剂+热解 | 300 360,500 300,500 300,400 380 120,430 | 180(反应时间) 39 60 30 360(反应时间) 60 | 无 无 无 ZSM-5 Al-Mg 无 | 无 无 无 无 无 Ca-C | 3.5 32.39 58.2 56.6~57.0 65.18 65~69 | 5.75 0.063 0.2 0.3 2.78 0 |
原料 | 脱氯方法 | 反应温度/℃ | 停留时间/min | 催化剂 | 吸附剂 | 油质量分数/% | 油中氯质量分数/% |
---|---|---|---|---|---|---|---|
PVC[ PVC[ PE\PP\PS\PVC\PET[ PE\PP\PS\PVC\PET[ PP\PVC[ PE\PP\PS\PVC[ | 热解 逐步热解 逐步热解 分步催化热解 催化热解 吸附剂+热解 | 300 360,500 300,500 300,400 380 120,430 | 180(反应时间) 39 60 30 360(反应时间) 60 | 无 无 无 ZSM-5 Al-Mg 无 | 无 无 无 无 无 Ca-C | 3.5 32.39 58.2 56.6~57.0 65.18 65~69 | 5.75 0.063 0.2 0.3 2.78 0 |
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